Geometric Optimization of Sonoreactors for the Enhancement of Sonochemical Activity

被引:71
|
作者
Son, Younggyu [2 ]
Lim, Myunghee [1 ]
Ashokkumar, Muthupandian [2 ]
Khim, Jeehyeong [1 ]
机构
[1] Korea Univ, Sch Civil Environm & Architectural Engn, Seoul 136701, South Korea
[2] Univ Melbourne, Sch Chem, Melbourne, Vic 3010, Australia
来源
JOURNAL OF PHYSICAL CHEMISTRY C | 2011年 / 115卷 / 10期
关键词
HIGH-FREQUENCY; DEGRADATION; SONOLUMINESCENCE; ULTRASOUND; INTENSITY; SONOCHEMILUMINESCENCE; REACTORS; SCIENCE; BUBBLES; POWER;
D O I
10.1021/jp110319y
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Acoustic cavitation concentrates and releases a very large amount of energy in localized areas, which can be used for many physical and chemical processes. Even though acoustic cavitation has been studied widely for decades, only few studies have been devoted to optimization of medium to large scale reactors. In this study, the effect of ultrasound irradiation distance on the sonochemical activity has been investigated in 36 and 108 kHz cylindrical sonoreactors with various liquid heights ranging from 80 to 340 mm. As the liquid height/irradiation distance is increased, the cavitation yield increases significantly under the approximately same input energy conditions. The sonochemiluminescence (SCL) images for the visualization of the cavitation field also show that a stronger and more stable standing wave field is formed with higher SCL activity at higher liquid heights.
引用
收藏
页码:4096 / 4103
页数:8
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