Spin-liquid ground state in the frustrated kagome antiferromagnet MgCu3(OH)6Cl2

被引:59
|
作者
Kermarrec, E. [1 ]
Mendels, P. [1 ]
Bert, F. [1 ]
Colman, R. H. [2 ]
Wills, A. S. [2 ]
Strobel, P. [3 ]
Bonville, P. [4 ]
Hillier, A. [6 ]
Amato, A. [5 ]
机构
[1] Univ Paris 11, Phys Solides Lab, UMR CNRS 8502, F-91405 Orsay, France
[2] UCL, Dept Chem, London WC1H 0AJ, England
[3] Univ Grenoble 1, CNRS, Inst Neel, F-38042 Grenoble, France
[4] CE Saclay, Serv Phys Etat Condense, CEA CNRS, F-91191 Gif Sur Yvette, France
[5] Paul Scherrer Inst, Lab Muon Spin Spect, CH-5232 Villigen, Switzerland
[6] Rutherford Appleton Lab, ISIS Facil, Didcot OX11 OQX, Oxon, England
来源
PHYSICAL REVIEW B | 2011年 / 84卷 / 10期
关键词
ZNCU3(OH)(6)CL-2; RELAXATION;
D O I
10.1103/PhysRevB.84.100401
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We report muon spin resonance experiments on MgxCu4-x(OH)(6)Cl-2 with x similar to 1, a material isostructural to Herbertsmithite exhibiting regular kagome planes of S = 1/2 ions (Cu2+), and therefore a candidate for a spin-liquid ground state. We evidence the absence of any magnetic ordering down to 20 mK (similar to J/10(4)). We present a detailed investigation of the spin dynamics on well-characterized samples in zero and applied longitudinal fields, and a defect-based interpretation is proposed to explain the unconventional dynamics observed in the quantum spin-liquid phase.
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收藏
页数:5
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