STRUCTURE AND ELECTROCHEMICAL PROPERTIES OF COPPER(II) COORDINATION POLYMERS WITH LIGANDS CONTAINING NAPHTHYL AND ANTHRACYL FRAGMENTS

被引：5

作者：

Dorofeeva, V. N. ^{[1
]}

Mishura, A. M. ^{[1
]}

Lytvynenko, A. S. ^{[1
]}

Grabovaya, N. V. ^{[1
]}

Kiskin, M. A. ^{[2
]}

Kolotilov, S. V. ^{[1
]}

Eremenko, I. L. ^{[2
]}

Novotortsev, V. M. ^{[2
]}

机构：

[1] LV Pisarzhevskii Inst Phys Chem, Prospekt Nauky 31, UA-03028 Kiev, Ukraine

[2] NS Kurnakov Gen & Inorgan Chem Inst, Leninsky Prospekt 31,GSP-1, Moscow 119991, Russia

来源：

THEORETICAL AND EXPERIMENTAL CHEMISTRY | 2016年 / 52卷 / 02期

关键词：

porous coordination polymers; naphthyl; anthracyl; electrochemical reduction; cyclic voltammetry; modified electrodes; density functional theory;

D O I：

10.1007/s11237-016-9458-6

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

The potentials for the electrochemical reduction of glassy carbon electrodes with deposited copper(II) coordination polymers (CP) containing polypyridine ligands with naphthyl and anthracyl substituents are similar to the potentials of the redox transformations of the corresponding ligands. The difference between the reduction potential of the CP-modified electrode and the potential for the redox transformation of the ligands in solution is greater when the lowest unoccupied molecular orbital of the ligand is predominantly located not on the carbocyclic but rather heterocyclic fragment.

引用

页码：111 / 118

页数：8

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