High-Performance Next-Generation Perovskite Nanocrystal Scintillator for Nondestructive X-Ray Imaging

被引:367
|
作者
Heo, Jin Hyuck [1 ]
Shin, Dong Hee [1 ]
Park, Jin Kyoung [1 ]
Kim, Do Hun [1 ]
Lee, Sang Jin [1 ]
Im, Sang Hyuk [1 ]
机构
[1] Korea Univ, Dept Chem & Biol Engn, 145 Anam Ro, Seoul 17104, South Korea
基金
新加坡国家研究基金会;
关键词
cesium lead tribromide; nanocrystals; perovskite; scintillators; X-ray imaging; LIGHT YIELD; DETECTORS; EMISSION; CSPBBR3; CSI(TL);
D O I
10.1002/adma.201801743
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Readily commercializable and cost-effective next-generation CsPbBr3 perovskite nanocrystals (PNCs) based X-ray detectors are demonstrated. The PNCs-based X-ray detector exhibits higher spatial resolution (9.8 lp mm(-1) at modulation transfer function (MTF) = 0.2 and 12.5-8.9 lp mm(-1) for a linear line chart), faster response time (approximate to 200 ns), and comparable stability (>40 Gy(air) s(-1) of X-ray exposure) compared with the commercialized terbium-doped gadolinium oxysulfide (GOS)-based detectors (spatial resolution = 6.2 lp mm(-1) at MTF = 0.2 and 6.3 lp mm(-1) for a linear line chart, response time = approximate to 1200 ns) because the PNCs-based scintillator has approximate to 5.6-fold faster average photoluminescence lifetime and stronger emission than the GOS-based one.
引用
收藏
页数:6
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