Disordered hyperuniformity in two-dimensional amorphous silica

被引:53
|
作者
Zheng, Yu [1 ]
Liu, Lei [2 ]
Nan, Hanqing [2 ]
Shen, Zhen-Xiong [3 ,4 ]
Zhang, Ge [5 ]
Chen, Duyu [6 ]
He, Lixin [3 ,4 ]
Xu, Wenxiang [2 ,7 ]
Chen, Mohan [8 ]
Jiao, Yang [1 ,2 ]
Zhuang, Houlong [1 ,2 ]
机构
[1] Arizona State Univ, Dept Phys, Tempe, AZ 85287 USA
[2] Arizona State Univ, Sch Engn Matter Transport & Energy, Tempe, AZ 85287 USA
[3] Univ Sci & Technol China, Key Lab Quantum Informat, Hefei 230026, Anhui, Peoples R China
[4] Univ Sci & Technol China, Synerget Innovat Ctr Quantum Informat & Quantum P, Hefei 230026, Anhui, Peoples R China
[5] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA
[6] Carnegie Mellon Univ, Tepper Sch Business, Pittsburgh, PA 15213 USA
[7] Hohai Univ, Coll Mech & Mat, Nanjing 211100, Peoples R China
[8] Peking Univ, HEDPS, CAPT, Coll Engn, Beijing 100871, Peoples R China
关键词
GLASS;
D O I
10.1126/sciadv.aba0826
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Disordered hyperuniformity (DHU) is a recently proposed new state of matter, which has been observed in a variety of classical and quantum many-body systems. DHU systems are characterized by vanishing infinite-wavelength normalized density fluctuations and are endowed with unique novel physical properties. Here, we report the discovery of disordered hyperuniformity in atomic-scale two-dimensional materials, i.e., amorphous silica composed of a single layer of atoms, based on spectral-density analysis of high-resolution transmission electron microscopy images. Moreover, we show via large-scale density functional theory calculations that DHU leads to almost complete closure of the electronic bandgap compared to the crystalline counterpart, making the material effectively a metal. This is in contrast to the conventional wisdom that disorder generally diminishes electronic transport and is due to the unique electron wave localization induced by the topological defects in the DHU state.
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页数:5
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