Hydrogen production of solar-driven steam gasification of sewage sludge in an indirectly irradiated fluidized-bed reactor

被引:28
|
作者
Li, Xian [1 ]
Shen, Ye [1 ]
Wei, Liping [1 ]
He, Chao [2 ]
Lapkin, Alexei A. [3 ,4 ]
Lipinski, Wojciech [5 ]
Dai, Yanjun [6 ]
Wang, Chi-Hwa [7 ]
机构
[1] Natl Univ Singapore, NUS Environm Res Inst, Singapore 138602, Singapore
[2] Nanyang Technol Univ, Sch Chem & Biomed Engn, 62 Nanyang Dr, Singapore 637459, Singapore
[3] Cambridge Ctr Adv Res & Educ Singapore Ltd, 1 Create Way,CREATE Tower 05-05, Singapore 138602, Singapore
[4] Univ Cambridge, Dept Chem Engn & Biotechnol, Philippa Fawcett Dr, Cambridge CB3 0AS, England
[5] Australian Natl Univ, Res Sch Elect Energy & Mat Engn, Canberra, ACT 2601, Australia
[6] Shanghai Jiao Tong Univ, Sch Mech Engn, Shanghai 200240, Peoples R China
[7] Natl Univ Singapore, Dept Chem & Biomol Engn, Singapore 117585, Singapore
基金
新加坡国家研究基金会;
关键词
Steam gasification; Fluidized bed; Sewage sludge; Concentrated solar radiation; Solar-to-fuel efficiency; Solar upgraded ratio; BUBBLE DIAMETER; KINETIC-MODEL; HEAT-TRANSFER; COAL COKES; BIOMASS; SYNGAS; TUBE; GAS; PYROLYSIS; DESIGN;
D O I
10.1016/j.apenergy.2019.114229
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
A fluidized-bed based solar steam gasification of sewage sludge for production of high-quality syngas with a high content of hydrogen is numerically modeled and validated by experimental data generated from a lab-scale fluidized bed. The solar gasifier is mainly composed of a fluidized bed and a concentrically tubular cavity. A transient model coupling a two-phase fluidization model (in terms of reaction kinetics and hydrodynamics) and a solar cavity receiver model is established to conduct the parametric investigation of the proposed solar gasifier, including the effects of the direct normal irradiance, gasifying agent composition, and spatial flux distribution at the freeboard wall on the performance criteria of solar gasification i.e. solar upgraded ratio and solar-to-fuel efficiency. The transient simulation of the solar gasifier with similar to 2.2 MW solar power input is performed. A H-2 yield range of 61.2-67.6 g/kg(sludge) can be achieved through solar steam gasification of sewage sludge, which can be adjusted by modifying the steam content of the gasifying agent and the direct normal irradiance. Under the condition of the direct normal irradiation of 1000 W/m(2), the mean concentration ratio of 1000 suns at the dense bed, and 100 vol% N-2 content, a maximum solar upgraded ratio of 1.0 and solar-to-fuel efficiency of 0.26 can be achieved.
引用
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页数:17
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