Bright and Efficient Full-Color Colloidal Quantum Dot Light-Emitting Diodes Using an Inverted Device Structure

被引:782
|
作者
Kwak, Jeonghun [5 ]
Bae, Wan Ki [4 ]
Lee, Donggu [2 ]
Park, Insun [3 ]
Lim, Jaehoon [1 ]
Park, Myeongjin [2 ]
Cho, Hyunduck [2 ]
Woo, Heeje [1 ]
Yoon, Do Y. [3 ]
Char, Kookheon [1 ]
Lee, Seonghoon [3 ]
Lee, Changhee [2 ]
机构
[1] Seoul Natl Univ, Sch Chem & Biol Engn, Seoul 151744, South Korea
[2] Seoul Natl Univ, Inter Univ Semicond Res Ctr, Sch Elect & Comp Engn, Seoul 151744, South Korea
[3] Seoul Natl Univ, Dept Chem, Seoul 151744, South Korea
[4] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA
[5] Dong A Univ, Dept Elect Engn, Pusan 604714, South Korea
基金
新加坡国家研究基金会;
关键词
Quantum dots; quantum dot light-emitting diodes; inverted device structure; electroluminescence; zinc oxide nanoparticles; ELECTROLUMINESCENCE; NANOCRYSTALS; ZNO; GREEN;
D O I
10.1021/nl3003254
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
We report highly bright and efficient inverted structure quantum dot (QD) based light-emitting diodes (QLEDs) by using solution-processed ZnO nanoparticles as the electron injection/transport layer and by optimizing energy levels with the organic hole transport layer. We have successfully demonstrated highly bright red, green, and blue QLEDs showing maximum luminances up to 23 040, 218 800, and 2250 cd/m(2), and external quantum efficiencies of 7.3, 5.8, and 1.7%, respectively. It is also noticeable that they showed turn-on voltages as low as the bandgap energy of each QD and long operational lifetime, mainly attributed to the direct exciton recombination within QDs through the inverted device structure. These results signify a remarkable progress in QLEDs and offer a practicable platform for the realization of QD-based full-color displays and lightings.
引用
收藏
页码:2362 / 2366
页数:5
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