One-step synthesis of Ag3VO4/diatomite composite material for efficient degradation of organic dyes under visible light

被引:8
|
作者
Zhu, Haitao [1 ,4 ]
Ren, Qifang [4 ,5 ,6 ]
Ding, Yi [1 ,4 ,5 ]
Zhu, Changhu [4 ]
Zong, Yixuan [4 ]
Hu, Xiaoye [2 ,3 ]
Jin, Zhen [1 ,4 ,5 ]
机构
[1] Anhui Jianzhu Univ, Anhui Adv Bldg Mat Engn Lab, Hefei 230601, Anhui, Peoples R China
[2] Chinese Acad Sci, Inst Solid State Phys, Key Lab Mat Phys, Hefei 230031, Anhui, Peoples R China
[3] Chinese Acad Sci, Inst Solid State Phys, Anhui Key Lab Nanomat & Nanostruct, Hefei 230031, Anhui, Peoples R China
[4] Anhui Jianzhu Univ, Sch Mat & Chem Engn, Hefei 230601, Anhui, Peoples R China
[5] Anhui Adv Bldg Mat Engn Lab, Hefei 230601, Anhui, Peoples R China
[6] Anhui Prov Int Res Ctr Adv Bldg Mat, Hefei 230601, Anhui, Peoples R China
基金
中国国家自然科学基金;
关键词
Ag3VO4; Diatomite; Photodegradation; Visible-light driven; ENHANCED PHOTOCATALYTIC ACTIVITY; HETEROJUNCTION PHOTOCATALYSTS; POROUS DIATOMITE; DRIVEN; PERFORMANCE; CONSTRUCTION; FABRICATION; POLLUTANTS; NANOSHEETS; TIO2;
D O I
10.1016/j.inoche.2021.108759
中图分类号
O61 [无机化学];
学科分类号
070301 ; 081704 ;
摘要
In this work, the Ag3VO4/diatomite composites with different ratio were successfully synthesized through one-step method. Through relevant characterizations, the results indicated that a large number of Ag3VO4 nanoparticles attached to the surface and pores in the diatomite. The photocatalytic performances of the samples were analyzed using degradation of RhB in aqueous solution under visible light irradiation (lambda >= 400 nm). The results showed that the Ag3VO4/diatomite composite exhibited the highest photocatalytic activity when the diatomite content reached 50%. After 40 min irradiation, almost 96% of RhB can be degraded. The photodynamic kinetic constant of the 50%-Ag3VO4/diatomite composite is 3.57 times higher than that of pure Ag3VO4 nanoparticles. In addition, the photocatalyst can be repetitively used with a high photocatalytic activity. The photocatalytic mechanism also has been discussed. It is believed that the Ag3VO4/diatomite composites have extensive potential applications in waste water treatment.
引用
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页数:9
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