Evaluation of visible photocatalytic performance of microwave hydrothermal synthesis of MnO2/TiO2 core-shell structures and gaseous mercury removal

被引:17
|
作者
Xie, Cheng [1 ,4 ]
Xu, Lei [1 ,4 ]
Xia, Yi [2 ,3 ]
Gang, Ruiqi [1 ,4 ]
Ye, Qianjun [1 ,4 ]
Koppala, Sivasankar [1 ,4 ,5 ]
机构
[1] Kunming Univ Sci & Technol, Fac Met & Energy Engn, Natl Local Joint Lab Engn Applicat Microwave Ener, Kunming 650093, Yunnan, Peoples R China
[2] Kunming Univ Sci & Technol, Res Ctr Anal & Measurement, Kunming 650093, Yunnan, Peoples R China
[3] Analyt & Testing Res Ctr Yunnan, Kunming 650093, Yunnan, Peoples R China
[4] Minist Educ, Key Lab Unconvent Met, Kunming 650093, Yunnan, Peoples R China
[5] Saveetha Inst Med & Tech Sci SIMATS, Saveetha Sch Engn, Chennai 602105, Tamil Nadu, India
基金
国家重点研发计划; 中国国家自然科学基金;
关键词
Core-shell structure; TiO2; MnO2; RhB degradation; Hg-0; removal; TIO2; HETEROJUNCTION; HETEROSTRUCTURE; NANOCOMPOSITE; CONSTRUCTION; FABRICATION; HYBRIDS;
D O I
10.1016/j.micromeso.2022.111788
中图分类号
O69 [应用化学];
学科分类号
081704 ;
摘要
MnO2/TiO2 core-shell structure photocatalyst was prepared by a two-step microwave method. Under visible light irradiation, this core-shell photocatalyst exhibited enhanced catalytic activity for the degradation of organic dye Rhodamine B and the oxidative removal of gaseous heavy metal He . The MnO2 shell not only enhanced the visible light absorption of TiO2, but also increased its specific surface area to 227.94 m(2) g(-1). In addition, the formation of core-shell heterojunction promotes the migration of carriers and the separation of photo-generated electron-hole pairs, and improves the stability of the composite, thus enabling it to exhibit enhanced photocatalytic performance.
引用
收藏
页数:10
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