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Evaluation of visible photocatalytic performance of microwave hydrothermal synthesis of MnO2/TiO2 core-shell structures and gaseous mercury removal
被引:17
|作者:
Xie, Cheng
[1
,4
]
Xu, Lei
[1
,4
]
Xia, Yi
[2
,3
]
Gang, Ruiqi
[1
,4
]
Ye, Qianjun
[1
,4
]
Koppala, Sivasankar
[1
,4
,5
]
机构:
[1] Kunming Univ Sci & Technol, Fac Met & Energy Engn, Natl Local Joint Lab Engn Applicat Microwave Ener, Kunming 650093, Yunnan, Peoples R China
[2] Kunming Univ Sci & Technol, Res Ctr Anal & Measurement, Kunming 650093, Yunnan, Peoples R China
[3] Analyt & Testing Res Ctr Yunnan, Kunming 650093, Yunnan, Peoples R China
[4] Minist Educ, Key Lab Unconvent Met, Kunming 650093, Yunnan, Peoples R China
[5] Saveetha Inst Med & Tech Sci SIMATS, Saveetha Sch Engn, Chennai 602105, Tamil Nadu, India
基金:
国家重点研发计划;
中国国家自然科学基金;
关键词:
Core-shell structure;
TiO2;
MnO2;
RhB degradation;
Hg-0;
removal;
TIO2;
HETEROJUNCTION;
HETEROSTRUCTURE;
NANOCOMPOSITE;
CONSTRUCTION;
FABRICATION;
HYBRIDS;
D O I:
10.1016/j.micromeso.2022.111788
中图分类号:
O69 [应用化学];
学科分类号:
081704 ;
摘要:
MnO2/TiO2 core-shell structure photocatalyst was prepared by a two-step microwave method. Under visible light irradiation, this core-shell photocatalyst exhibited enhanced catalytic activity for the degradation of organic dye Rhodamine B and the oxidative removal of gaseous heavy metal He . The MnO2 shell not only enhanced the visible light absorption of TiO2, but also increased its specific surface area to 227.94 m(2) g(-1). In addition, the formation of core-shell heterojunction promotes the migration of carriers and the separation of photo-generated electron-hole pairs, and improves the stability of the composite, thus enabling it to exhibit enhanced photocatalytic performance.
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页数:10
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