X-ray absorption spectroscopy using a self-seeded soft X-ray free-electron laser

被引：16

作者：

Kroll, Thomas ^{[1
,2
]}

Kern, Jan ^{[1
,3
]}

Kubin, Markus ^{[4
]}

Ratner, Daniel ^{[1
]}

Gul, Sheraz ^{[3
]}

Fuller, Franklin D. ^{[3
]}

Loechel, Heike ^{[5
]}

Krzywinski, Jacek ^{[1
]}

Lutman, Alberto ^{[1
]}

Ding, Yuantao ^{[1
]}

Dakovski, Georgi L. ^{[1
]}

Moeller, Stefan ^{[1
]}

Turner, Joshua J. ^{[1
]}

Alonso-Mori, Roberto ^{[1
]}

Nordlund, Dennis L. ^{[2
]}

Rehanek, Jens ^{[5
,6
]}

Weniger, Christian ^{[4
]}

Firsov, Alexander ^{[5
]}

Brzhezinskaya, Maria ^{[5
]}

Chatterjee, Ruchira ^{[3
]}

Lassalle-Kaiser, Benedikt ^{[7
]}

Sierra, Raymond G. ^{[1
,8
]}

Laksmono, Hartawan ^{[8
]}

Hill, Ethan ^{[9
]}

Borovik, Andrew ^{[9
]}

Erko, Alexei ^{[5
]}

Foehlisch, Alexander ^{[4
,10
]}

Mitzner, Rolf ^{[4
]}

Yachandra, Vittal K. ^{[3
]}

Yano, Junko ^{[3
]}

Wernet, Philippe ^{[4
]}

Bergmann, Uwe ^{[1
,8
]}

机构：

[1] SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA 94025 USA

[2] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA

[3] Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, Berkeley, CA 94720 USA

[4] Helmholtz Zentrum Berlin Mat & Energie GmbH, Inst Methods & Instrumentat Synchrotron Rad, D-12489 Berlin, Germany

[5] Helmholtz Zentrum Berlin Mat & Energie, Inst Nanometer Opt & Technol, D-12489 Berlin, Germany

[6] Paul Scherrer Inst, CH-5232 Villigen, Switzerland

[7] Synchrotron SOLEIL, St Aubin BP 48, F-91192 Gif Sur Yvette, France

[8] SLAC Natl Accelerator Lab, Stanford PULSE Inst, Menlo Pk, CA 94025 USA

[9] Univ Calif Irvine, Dept Chem, 1102 Nat Sci 2, Irvine, CA 92697 USA

[10] Univ Potsdam, Inst Phys & Astron, Karl Liebknecht Str 24-25, D-14476 Potsdam, Germany

来源：

OPTICS EXPRESS | 2016年 / 24卷 / 20期

基金：

美国国家卫生研究院;

关键词：

COHERENT-LIGHT SOURCE; EMISSION-SPECTROSCOPY; DYNAMICS; PULSE; INSTRUMENT; OXIDATION; GRATINGS; SCIENCE;

D O I：

10.1364/OE.24.022469

中图分类号：

O43 [光学];

学科分类号：

070207 ; 0803 ;

摘要：

X-ray free electron lasers (XFELs) enable unprecedented new ways to study the electronic structure and dynamics of transition metal systems. L-edge absorption spectroscopy is a powerful technique for such studies and the feasibility of this method at XFELs for solutions and solids has been demonstrated. However, the required x-ray bandwidth is an order of magnitude narrower than that of self-amplified spontaneous emission (SASE), and additional monochromatization is needed. Here we compare L-edge x-ray absorption spectroscopy (XAS) of a prototypical transition metal system based on monochromatizing the SASE radiation of the linac coherent light source (LCLS) with a new technique based on self-seeding of LCLS. We demonstrate how L-edge XAS can be performed using the self-seeding scheme without the need of an additional beam line monochromator. We show how the spectral shape and pulse energy depend on the undulator setup and how this affects the x-ray spectroscopy measurements. (C) 2016 Optical Society of America

引用

页码：22469 / 22480

页数：12

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