Multiphoton antiresonance in large-spin systems

We study nonlinear response of a spin S > 1/2 with easy-axis anisotropy. The response displays sharp dips or peaks when the modulation frequency is adiabatically swept through multiphoton resonance. The effect is a consequence of a special symmetry of the spin dynamics in a magnetic field for the anisotropy energy proportional to S(z)(2). The occurrence of the dips or peaks is determined by the spin state. Their shape strongly depends on the modulation amplitude. Higher-order anisotropy breaks the symmetry, leading to sharp steps in the response as function of frequency. The results bear on the dynamics of molecular magnets in a static magnetic field.