Enhanced thermoelectric power in two-dimensional transition metal dichalcogenide monolayers

被引:77
|
作者
Pu, Jiang [1 ]
Kanahashi, Kaito [1 ]
Nguyen Thanh Cuong [2 ]
Chen, Chang-Hsiao [3 ]
Li, Lain-Jong [4 ]
Okada, Susumu [5 ,6 ]
Ohta, Hiromichi [7 ]
Takenobu, Taishi [1 ,8 ]
机构
[1] Waseda Univ, Dept Adv Sci & Engn, Tokyo 1698555, Japan
[2] Natl Inst Mat Sci, ICYS, Tsukuba, Ibaraki 3050044, Japan
[3] Natl Inst Mat Sci, Int Ctr Mat Nanoarchitecton MANA, Tsukuba, Ibaraki 3050044, Japan
[4] Feng Chia Univ, Dept Automat Control Engn, Taichung 40724, Taiwan
[5] King Abdullah Univ Sci & Technol, Phys Sci & Engn Div, Thuwal 239556900, Saudi Arabia
[6] Univ Tsukuba, Grad Sch Pure & Appl Sci, Ibaraki 3058571, Japan
[7] Hokkaido Univ, Res Inst Elect Sci, Sapporo, Hokkaido 0010020, Japan
[8] Waseda Univ, Kagami Mem Lab Mat Sci & Technol, Tokyo 1690051, Japan
基金
日本学术振兴会;
关键词
CHEMICAL-VAPOR-DEPOSITION; QUANTUM-WELL STRUCTURES; SINGLE-CRYSTALS; THERMAL-CONDUCTIVITY; MOS2; TRANSISTORS; FIGURE; LAYERS; WS2;
D O I
10.1103/PhysRevB.94.014312
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The carrier-density-dependent conductance and thermoelectric properties of large-area MoS2 and WSe2 monolayers are simultaneously investigated using the electrolyte gating method. The sign of the thermoelectric power changes across the transistor off-state in the ambipolar WSe2 transistor as the majority carrier density switches from electron to hole. The thermopower and thermoelectric power factor of monolayer samples are one order of magnitude larger than that of bulk materials, and their carrier-density dependences exhibit a quantitative agreement with the semiclassical Mott relation based on the two-dimensional energy band structure, concluding the thermoelectric properties are enhanced by the low-dimensional effect.
引用
收藏
页数:8
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