2022 roadmap on low temperature electrochemical CO2 reduction

被引：125

作者：

Stephens, Ifan E. L. ^{[1
]}

Chan, Karen ^{[2
]}

Bagger, Alexander ^{[3
]}

Boettcher, Shannon W. ^{[4
,5
]}

Bonin, Julien ^{[6
]}

Boutin, Etienne ^{[7
]}

Buckley, Aya K. ^{[8
]}

Buonsanti, Raffaella ^{[9
]}

Cave, Etosha R. ^{[8
]}

Chang, Xiaoxia ^{[10
]}

Chee, See Wee ^{[11
]}

da Silva, Alisson H. M. ^{[12
]}

de Luna, Phil ^{[13
]}

Einsle, Oliver ^{[14
]}

Endrodi, Balazs ^{[15
]}

Escudero-Escribano, Maria ^{[3
]}

de Araujo, Jorge V. Ferreira ^{[16
]}

Figueiredo, Marta C. ^{[17
,22
]}

Hahn, Christopher ^{[18
]}

Hansen, Kentaro U. ^{[19
]}

Haussener, Sophia ^{[7
]}

Hunegnaw, Sara ^{[8
]}

Huo, Ziyang ^{[8
]}

Hwang, Yun Jeong ^{[20
,23
]}

Janaky, Csaba ^{[15
,21
]}

Jayathilake, Buddhinie S. ^{[18
]}

Jiao, Feng ^{[19
]}

Jovanov, Zarko P. ^{[16
]}

Karimi, Parisa ^{[13
]}

Koper, Marc T. M. ^{[12
]}

Kuhl, Kendra P. ^{[8
]}

Lee, Woong Hee ^{[20
,25
]}

Liang, Zhiqin ^{[12
]}

Liu, Xuan ^{[12
]}

Ma, Sichao ^{[8
]}

Ma, Ming ^{[24
]}

Oh, Hyung-Suk ^{[25
,26
]}

Robert, Marc ^{[6
,27
]}

Cuenya, Beatriz Roldan ^{[11
]}

Rossmeisl, Jan ^{[3
]}

Roy, Claudie ^{[13
]}

Ryan, Mary P. ^{[1
]}

Sargent, Edward H. ^{[28
]}

Sebastian-Pascual, Paula ^{[3
]}

Seger, Brian ^{[29
]}

Steier, Ludmilla ^{[1
,30
]}

Strasser, Peter ^{[31
]}

Varela, Ana Sofia ^{[32
]}

Vos, Rafael E. ^{[12
]}

Wang, Xue ^{[28
]}

机构：

[1] Imperial Coll London, Dept Mat, Exhibit Rd, London SW7 2AZ, England

[2] Tech Univ Denmark, Catalysis Theory Ctr, Dept Phys, DK-2800 Lyngby, Denmark

[3] Univ Copenhagen, Dept Chem, DK-2100 Copenhagen, Denmark

[4] Univ Oregon, Dept Chem & Biochem, Eugene, OR 97403 USA

[5] Univ Oregon, Oregon Ctr Electrochem, Eugene, OR 97403 USA

[6] Univ Paris Cite, Lab Electrochim Mol, CNRS, F-75006 Paris, France

[7] Ecole Polytech Fed Lausanne, Lab Renewable Energy Sci & Engn, CH-1015 Lausanne, Switzerland

[8] Twelve Benefit Corp, 614 Bancroft Way, Berkeley, CA 94710 USA

[9] Ecole Polytech Fed Lausanne, Inst Chem Sci & Engn, Lab Nanochem Energy LNCE, CH-1950 Sion, Switzerland

[10] Peking Univ, Coll Chem & Mol Engn, Beijing, Peoples R China

[11] Max Planck Gesell, Fritz Haber Inst, Dept Interface Sci, Faradayweg 4-6, D-14195 Berlin, Germany

[12] Leiden Inst Chem, Einsteinweg 55, NL-2333 CC Leiden, Netherlands

[13] Natl Res Council Canada, Energy Min & Environm Res Ctr, Ottawa, ON K1A 0R6, Canada

[14] Albert Ludwigs Univ Freiburg, Inst Biochem, D-79104 Freiburg, Germany

[15] Univ Szeged, Dept Phys Chem & Mat Sci, Rerrich Sq 1, H-6720 Szeged, Hungary

[16] Tech Univ Berlin, LIQUIDLOOP GmbH, Hardenbergstr 38,AM1, D-10623 Berlin, Germany

[17] Eindhoven Univ Technol, Chem Engn & Chem Dept, POB 513, NL-5600 MB Eindhoven, Netherlands

[18] Lawrence Livermore Natl Lab, Mat Sci Div, Livermore, CA 94550 USA

[19] Univ Delaware, Dept Chem & Biomol Engn, 150 Acad St, Newark, DE 19716 USA

[20] Seoul Natl Univ, Dept Chem, Seoul 08826, South Korea

[21] eChemicles Zrt, Also Kikoto Sor 11, H-6726 Szeged, Hungary

[22] Eindhoven Inst Renewable Energy Syst, POB 513, NL-5600 MB Eindhoven, Netherlands

[23] Inst Basic Sci IBS, Ctr Nanoparticle Res, Seoul 08826, South Korea

[24] Xi An Jiao Tong Univ, Sch Chem Engn & Technol, Xian 710049, Peoples R China

[25] Korea Inst Sci & Technol KIST, Clean Energy Res Ctr, Seoul 02792, South Korea

[26] Kyung Hee Univ, KHU KIST Dept Conversing Sci & Technol, Seoul 02447, South Korea

[27] Inst Univ France, F-75005 Paris, France

[28] Univ Toronto, Dept Elect & Comp Engn, Toronto, ON M5S 1A4, Canada

[29] Tech Univ Denmark, Dept Phys, Sect Surface Phys & Catalysis SurfCat, DK-2800 Lyngby, Denmark

[30] Univ Oxford, Dept Chem, Oxford, England

[31] Tech Univ Berlin, Dept Chem, Chem Engn Div, Str 17 Juni 124, D-10623 Berlin, Germany

[32] Univ Nacl Autonoma Mexico, Inst Chem, Mexico City, DF, Mexico

来源：

JOURNAL OF PHYSICS-ENERGY | 2022年 / 4卷 / 04期

基金：

加拿大自然科学与工程研究理事会;

关键词：

electrocatalysis; CO2; reduction; electrochemistry; solar fuels; CARBON-DIOXIDE CAPTURE; ELECTROCATALYTIC CONVERSION; SELECTIVE ELECTROREDUCTION; TECHNOECONOMIC ANALYSIS; ACCELERATED DISCOVERY; MECHANISTIC INSIGHTS; BIPOLAR MEMBRANES; METAL-ELECTRODES; STRUCTURAL BASIS; LIQUID FUEL;

D O I：

10.1088/2515-7655/ac7823

中图分类号：

TE [石油、天然气工业]; TK [能源与动力工程];

学科分类号：

0807 ; 0820 ;

摘要：

Electrochemical CO2 reduction (CO2R) is an attractive option for storing renewable electricity and for the sustainable production of valuable chemicals and fuels. In this roadmap, we review recent progress in fundamental understanding, catalyst development, and in engineering and scale-up. We discuss the outstanding challenges towards commercialization of electrochemical CO2R technology: energy efficiencies, selectivities, low current densities, and stability. We highlight the opportunities in establishing rigorous standards for benchmarking performance, advances in in operando characterization, the discovery of new materials towards high value products, the investigation of phenomena across multiple-length scales and the application of data science towards doing so. We hope that this collective perspective sparks new research activities that ultimately bring us a step closer towards establishing a low- or zero-emission carbon cycle.

引用

页数：84

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