Distribution characteristics and indicator significance of Dechloranes in multi-matrices at Ny-Alesund in the Arctic

被引:25
|
作者
Na, Guangshui [1 ,2 ]
Wei, Wei [1 ,3 ]
Zhou, Shiyao [5 ]
Gao, Hui [1 ]
Ma, Xindong [1 ]
Qiu, Lina [1 ,4 ]
Ge, Linke [1 ]
Bao, Chenguang [1 ]
Yao, Ziwei [1 ]
机构
[1] Natl Marine Environm Monitoring Ctr, Key Lab Ecol Environm Coastal Areas, Dalian 116023, Peoples R China
[2] Chinese Acad Sci, Res Ctr Ecoenvironm Sci, Beijing 100085, Peoples R China
[3] Liaoning Normal Univ, Sch Chem & Chem Engn, Dalian 116029, Peoples R China
[4] Dalian Polytech Univ, Sch Biol Technol, Dalian 116034, Peoples R China
[5] Dalian Inst Sci & Technol, Dalian 116052, Peoples R China
来源
基金
中国国家自然科学基金;
关键词
Dechloranes; Arctic; Multi-matrices; Distribution characteristic; Ratio; Source analysis; FLAME RETARDANTS; LAKE-ONTARIO; GREAT-LAKES; ISOMER PROFILES; SOUTH CHINA; PLUS; AIR; SEDIMENT; CANADA; BIOTA;
D O I
10.1016/j.jes.2014.07.019
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
In recent years, Dechloranes have been widely detected in the environment around the world. However, understanding and knowledge of Dechloranes in remote regions, such as the Arctic, remain lacking. Therefore, the concentrations of 5 Dechloranes in surface seawater, sediment, soil, moss, and dung collected from Ny-Alesund in the Arctic were measured with the concentrations 93 pg/L, 342, 325, 1.4, and 258 pg/g, respectively, which were much lower than those in Asian and European regions. The mean ratios of anti-Dechlorane Plus (DP) to total DP (f(anti)) in seawater, sediment, soil, moss, dung, and atmospheric samples were 0.36, 0.21, 0.18, 0.27, 0.66, and 0.43, respectively. Results suggested that the main source of DP in seawater, sediment, soil, and moss was long-range atmospheric transport. However, the ratio identified in dung was different, for which the migration behavior of the organism is probably the main source of DP. (C) 2014 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V.
引用
收藏
页码:8 / 13
页数:6
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