Frustration of direct photoionizations of rare gas clusters in intense extreme ultraviolet free-electron laser pulses

被引:4
|
作者
Iwayama, H. [1 ,3 ,7 ]
Nagaya, K. [1 ,7 ]
Murakami, H. [1 ,7 ]
Yao, M. [1 ,7 ]
Fukuzawa, H. [2 ,7 ]
Liu, X. J. [2 ,7 ]
Pruemper, G. [2 ,7 ]
Okunishi, M. [2 ]
Shimada, K. [2 ]
Ueda, K. [2 ,7 ]
Harada, T. [2 ]
Toyoda, M. [2 ]
Yanagihara, M. [2 ]
Yamamoto, M. [2 ]
Motomura, K. [2 ,7 ]
Saito, N. [3 ,7 ]
Rudenko, A. [4 ,7 ]
Ullrich, J. [4 ,5 ,7 ]
Foucar, L. [6 ,7 ]
Czasch, A. [6 ]
Doerner, R. [6 ]
Nagasono, M. [7 ]
Higashiya, A. [7 ]
Yabashi, M. [7 ]
Ishikawa, T. [7 ]
Ohashi, H. [7 ,8 ]
Kimura, H. [7 ,8 ]
Togashi, T. [7 ]
机构
[1] Kyoto Univ, Dept Phys, Kyoto 6068502, Japan
[2] Tohoku Univ, Inst Multidisciplinary Res Adv Mat, Sendai, Miyagi 9808577, Japan
[3] AIST, Natl Metrol Inst Japan, Tsukuba, Ibaraki 3058568, Japan
[4] CFel, Max Planck Adv Std Grp, D-22607 Hamburg, Germany
[5] Max Planck Inst Kernphys, D-69117 Heidelberg, Germany
[6] Goethe Univ Frankfurt, Inst Kernphys, D-60486 Frankfurt, Germany
[7] RIKEN, Mikazuki, Hyogo 6795148, Japan
[8] Japan Synchrotron Radiat Res Inst, Hyogo 6795198, Japan
关键词
MULTIPLE IONIZATION; ION;
D O I
10.1088/1742-6596/212/1/012014
中图分类号
O64 [物理化学(理论化学)、化学物理学]; O56 [分子物理学、原子物理学];
学科分类号
070203 ; 070304 ; 081704 ; 1406 ;
摘要
We performed a momentum imaging measurements of Ar clusters irradiated by extreme ultraviolet free electron laser pulses (61nm 1.3x10(11) W/cm(2)) for various cluster sizes. Dominant fragment ions were Ar+ and Ar-2(+) ions with significant kinetic energy (up to 40eV). This indicates that Ar clusters absorbed many photons, become highly ionized and finally dissociated into many fragments through Coulomb explosion. The size dependence of the ion kinetic energy distribution indicates that larger clusters significantly suffer from the frustration of direct photoelectron emissions and multiple ionizations.
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页数:5
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