Interfacial engineering of MoS2/TiO2 hybrids for enhanced electrocatalytic hydrogen evolution reaction

被引:26
|
作者
Song, Xiaolin [1 ]
Chen, Guifeng [1 ]
Guan, Lixiu [2 ]
Zhang, Hui [1 ]
Tao, Junguang [1 ]
机构
[1] Hebei Univ Technol, Sch Mat Sci & Engn, Key Lab New Type Funct Mat Hebei Prov, Tianjin 300130, Peoples R China
[2] Hebei Univ Technol, Sch Sci, Tianjin 300401, Peoples R China
关键词
ACTIVE EDGE SITES; PHOTOCATALYTIC ACTIVITIES; MOS2; TIO2; CATALYST; NANOSHEETS; CLEAVAGE; WATER;
D O I
10.7567/APEX.9.095801
中图分类号
O59 [应用物理学];
学科分类号
摘要
Herein, we show that the synergistic effect between MoS2 and TiO2 enhances the hydrogen evolution reaction ( HER) performance of their hybrids, which is tunable via interface engineering. Among several interfaces, MoS2/TiO2-H complexes exhibit the best HER activity. The observed Tafel slope of 66.9mV/dec is well in range of previous literature reports, suggesting a Volmer-Heyrovsky mechanism. Enhanced activities were attributed to abundant active sites at the interfaces, as well as improved charge transfer efficiency. Our results emphasize the roles that interfaces play in enhancing the HER activities of MoS2-based heterogeneous catalysts. (C) 2016 The Japan Society of Applied Physics
引用
收藏
页数:4
相关论文
共 50 条
  • [1] MoS2 nanotubes loaded with TiO2 nanoparticles for enhanced electrocatalytic hydrogen evolution
    Feng, Bo
    Liu, Chuntao
    Yan, Weiyi
    Geng, Jianxin
    Wang, Guimin
    [J]. RSC ADVANCES, 2019, 9 (45) : 26487 - 26494
  • [2] Electrocatalytic Hydrogen Evolution Study of MoS2 With Different Loading of TiO2 Nanoparticles
    Pal, Arnab
    Dutta, Shubhamita
    Jana, Tushar K.
    Chatterjee, Kuntal
    [J]. DAE SOLID STATE PHYSICS SYMPOSIUM 2018, 2019, 2115
  • [3] Facile synthesis of MoS2 nanosheets-deposited TiO2 nanotubes array electrode for enhanced electrocatalytic hydrogen evolution reaction
    Yousefzadeh, Samira
    Mardani, Nayyer
    [J]. INORGANIC CHEMISTRY COMMUNICATIONS, 2021, 127
  • [4] Well-patterned Au nanodots on MoS2/TiO2 hybrids for enhanced hydrogen evolution activity
    Tao, Junguang
    Chen, Shiqiang
    Guan, Lixiu
    Chen, Guifeng
    Yu, Chenqi
    Chen, Lei
    Cheng, Xiangrong
    Zhang, Hui
    Xie, Xinjian
    [J]. ELECTROCHIMICA ACTA, 2018, 283 : 419 - 427
  • [5] MoS2 compounded bidirectionally with TiO2 for hydrogen evolution reaction with enhanced humidity sensing performance
    Chen, Xiaofan
    Hu, Haoqi
    Feng, Yu
    Peng, Deyan
    Li, Bo
    Fu, Hao
    Guo, Bangjun
    Lei, Xiang
    Yu, Ke
    [J]. MATERIALS SCIENCE IN SEMICONDUCTOR PROCESSING, 2018, 82 : 75 - 81
  • [6] Engineering MoS2 for high-performance electrocatalytic hydrogen evolution
    Li, Guoqing
    Cao, Linyou
    [J]. ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2018, 255
  • [7] Synthesis of Ni-doped MoS2/graphene hybrids and their electrocatalytic activity for hydrogen evolution reaction
    Hou S.-C.
    Ren W.-Y.
    Zhu Q.
    Chen W.-X.
    [J]. Zhejiang Daxue Xuebao (Gongxue Ban)/Journal of Zhejiang University (Engineering Science), 2019, 53 (08): : 1610 - 1617
  • [8] Controlled Loading of MoS2 on Hierarchical Porous TiO2 for Enhanced Photocatalytic Hydrogen Evolution
    Tiwari, Amritanjali
    Gautam, Amit
    Sk, Saddam
    Gavali, Deepak S.
    Thapa, Ranjit
    Pal, Ujjwal
    [J]. JOURNAL OF PHYSICAL CHEMISTRY C, 2021, 125 (22): : 11950 - 11962
  • [9] MoS2 Nanosheet Loaded with TiO2 Nanoparticles: An Efficient Electrocatalyst for Hydrogen Evolution Reaction
    Shen, Yongzhen
    Ren, Xiaohui
    Qi, Xiang
    Zhou, Jie
    Huang, Zongyu
    Zhong, Jianxin
    [J]. JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2016, 163 (13) : H1087 - H1090
  • [10] Recent Modification Strategies of MoS2 for Enhanced Electrocatalytic Hydrogen Evolution
    Meng, Chao
    Chen, Xiaodong
    Gao, Yuanfeng
    Zhao, Qianqian
    Kong, Deqiang
    Lin, Mengchang
    Chen, Xuemin
    Li, Yuxia
    Zhou, Yue
    [J]. MOLECULES, 2020, 25 (05):