Catalytic conversion of CO2 to value added fuels: Current status, challenges, and future directions

被引:93
|
作者
Wu, Jingjie [1 ]
Zhou, Xiao-Dong [1 ]
机构
[1] Univ S Carolina, Dept Chem Engn, 301 Main St, Columbia, SC 29208 USA
关键词
Value added fuels; Electrocatalysts; Catalytic conversion; Carbon dioxide; Durability; CARBON-DIOXIDE REDUCTION; GAS-DIFFUSION ELECTRODES; COPPER SINGLE-CRYSTAL; HIGH-PRESSURE CO2; EFFICIENCY ELECTROCHEMICAL REDUCTION; FORMIC-ACID; PHOTOELECTROCHEMICAL REDUCTION; PULSED ELECTROREDUCTION; METAL-ELECTRODES; LOW-TEMPERATURE;
D O I
10.1016/S1872-2067(16)62455-5
中图分类号
O69 [应用化学];
学科分类号
081704 ;
摘要
The electrochemical reduction of CO2 into liquid fuels especially coupling with the intermittent renewable electricity offers a promising means of storing electricity in chemical form, which reduces the dependence on fossil fuels and mitigates the negative impact of anthropogenic CO2 emissions on the planet. Although converting CO2 to fuels is not in itself a new concept, the field has not substantially advanced in the last 30 years primarily because of the challenge of discovery of structural electrocatalysts and the development of membrane architectures for efficient collection of reactants and separation of products. This overview summarizes recent advances in catalytic conversion of CO2 and presents the challenges and future directions in producing value-added fuels. (C) 2016, Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. All rights reserved.
引用
收藏
页码:999 / 1015
页数:17
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