Stimulated Raman adiabatic passage in an extended ladder system

被引:9
|
作者
Niu, Ying-Yu [1 ]
Wang, Rong [1 ]
Qiu, Ming-Hui [1 ]
机构
[1] Dalian Jiaotong Univ, Sch Sci, Dalian 116028, Peoples R China
来源
PHYSICAL REVIEW A | 2011年 / 84卷 / 02期
基金
美国国家科学基金会;
关键词
POPULATION TRANSFER; DIATOMIC-MOLECULES; PULSE SEQUENCES; DISSOCIATION; EXCITATION;
D O I
10.1103/PhysRevA.84.023406
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
The rovibrational dynamics of an extended ladder stimulated Raman adiabatic passage (STIRAP) system through permanent dipole moment transitions is investigated theoretically using the time-dependent quantum-wave-packet method for the ground electronic state of the HF molecule. The calculated results show that nearly 100% of the population can be transferred to the target state through (1+2), (1+3), and (2+2) STIRAP schemes. By choosing a suitable excitation pathway, the effects of the background states on the final population of the target state can be removed. For the multiphoton STIRAP process, the one-photon overtone pump scheme is more efficient than the two-photon pump scheme in controlling the population transfer to the target state.
引用
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页数:5
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