Quantitative prediction of two-photon absorption cross section based on linear spectroscopic properties

被引：48

作者：

Rebane, Aleksander ^{[2
,3
]}

Makarov, Nikolay S. ^{[2
]}

Drobizhev, Mikhail ^{[2
]}

Spangler, Brenda ^{[1
]}

Tarter, E. Scott ^{[1
]}

Reeves, Benjamin D. ^{[1
]}

Spangler, Charles W. ^{[4
,5
]}

Meng, Fanqing

Suo, Zhiyong ^{[2
]}

机构：

[1] Sensopath Technol Inc, Bozeman, MT 59715 USA

[2] Montana State Univ, Dept Phys, Bozeman, MT 59717 USA

[3] NICPB, EE-12618 Tallinn, Estonia

[4] Montana State Univ, Dept Chem & Biochem, Bozeman, MT 59717 USA

[5] MPA Technol Inc, Bozeman, MT 59715 USA

来源：

JOURNAL OF PHYSICAL CHEMISTRY C | 2008年 / 112卷 / 21期

关键词：

D O I：

10.1021/jp800104q

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

We study two-photon absorption (2PA) spectra in a broad class of organic dye molecules, such as substituted diphenylaminostilbenes, push-pull porphyrins, and carbazol-substituted stilbenes. We show, for the first time, that the 2PA cross section in the lowest-energy dipole-allowed transition may be predicted with better than 50% absolute accuracy based solely on the molecular parameters obtained from linear spectroscopic measurements.

引用

页码：7997 / 8004

页数：8

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