Angle-resolved photoemission spectroscopy (ARPES) of Na0.7CoO2

被引:0
|
作者
Kuprin, A [1 ]
Hasan, Z
Chuang, YD
Hussain, Z
Qian, D
Foo, M
Cava, RJ
机构
[1] Princeton Univ, Dept Phys, Joseph Henry Labs, Princeton, NJ 08544 USA
[2] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA
[3] Princeton Mat Inst, Princeton Ctr Copplex Mat, Princeton, NJ 08544 USA
[4] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA
来源
关键词
cobalt oxyhydrates; Mott insulator; electron correlations; photoelectron spectroscopy;
D O I
10.1142/S0217979205028554
中图分类号
O59 [应用物理学];
学科分类号
摘要
Detailed study of the electronic structure of the layered Na0.7CoO2, doped Mott insulator with triangular Co lattice is performed by angle-resolved photoemission spectroscopy (ARPES). At low temperature Fermi surface is a centered hole pocket of hexagonal character shape in agreement with LDA. A broad valence band satellite at higher energies showing resonant enhancement at the 2p, 3p -> 3d excitations indicates large on-site Hubbard-U similar to 5 eV. A momentum dependent quasiparticle band near Fermi level that is flat and vanished at energies already above 70 meV or 80 meV gives a value of the single particle hopping t < 10 meV. This band is defined only in the region of non - Fermi liquid transport with linear growth of resistivity up to 120 K.
引用
收藏
页码:345 / 351
页数:7
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