Synthesis and photocatalytic performance of TiO2 spheres on ZnO arrays

被引:3
|
作者
Ren, Yuanwen [1 ]
Xia, Zelin [1 ]
Yu, Yue [1 ]
Bai, Xueying [1 ]
Liang, Yao [1 ]
Wang, Hualin [1 ]
Wang, Nan [1 ]
Jiang, Weiwei [1 ]
Liu, Shimin [1 ]
Liu, Chaoqian [1 ]
Ding, Wanyu [1 ]
Zhang, Zhihua [1 ]
Dong, Chuang [1 ]
机构
[1] Dalian Jiaotong Univ, Engn Res Ctr Optoelect Mat & Devices, Sch Mat Sci & Engn, Dalian 116028, Peoples R China
基金
中国国家自然科学基金;
关键词
ZnO; TiO2; Sphere; Calcination; Photocatalytic; THIN-FILMS; PHOTODEGRADATION; NANOPARTICLES; DEGRADATION; FABRICATION; ADSORPTION; CONVERSION; NANOSHEETS; SURFACE;
D O I
10.1016/j.optmat.2022.112440
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
TiO2 spheres were synthesized on ZnO arrays with Al doped ZnO (AZO) glass substrate (named as AZT) by a twostep method. XRD, SEM, EDS, TEM, and UV-Vis were used to explore the effect of calcination temperature on the crystal structure, morphology, composition and photocatalytic performance of AZT samples. Results indicate that the calcination temperature has a vital role in forming different morphologies of TiO2 including flake-like, block, spheres, and aggregates. The diameter of TiO2 spheres is in the range of 0.5-3.5 mu m, which increases first and then decreases with calcination temperature achieving a maximum at 450 degrees C. The sample calcined at 400 degrees C shows the most excellent photocatalytic degradation performance of methyl orange under 15 W weak-ultraviolet light irradiation, which is mainly due to the moderate particle size, high dispersibility and well crystallinity of TiO2 spheres.
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页数:8
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