Glass Transition of the Monodisperse Gaussian Core Model

被引:78
|
作者
Ikeda, Atsushi [1 ]
Miyazaki, Kunimasa [1 ]
机构
[1] Univ Tsukuba, Inst Phys, Tsukuba, Ibaraki 3058571, Japan
关键词
LENNARD-JONES MIXTURE; COUPLING THEORY; HETEROGENEOUS DYNAMICS; SUPERCOOLED LIQUIDS; SYSTEM; FLUID;
D O I
10.1103/PhysRevLett.106.015701
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We numerically investigate the dynamical properties of the one-component Gaussian core model in supercooled states. We find that nucleation is increasingly suppressed with increasing density. The system concomitantly exhibits glassy, slow dynamics characterized by the two-step stretched exponential relaxation of the density correlation and a drastic increase of the relaxation time. We also find a weaker violation of the Stokes-Einstein relation and a smaller non-Gaussian parameter than in typical model glass formers, implying weaker dynamic heterogeneities. Additionally, the agreement of the simulation data with the prediction of mode-coupling theory is exceptionally good, indicating that the nature of the slow dynamics of this ultrasoft particle fluid is mean-field-like. This fact may be understood as a consequence of the long-range nature of the interaction.
引用
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页数:4
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