Involvement of Surface-Bound Radicals in the Oxidation of Toluene Using Supported Au-Pd Nanoparticles

被引:86
|
作者
bin Saiman, Mohd Izham [1 ]
Brett, Gemma L. [1 ]
Tiruvalam, Ramchandra [2 ]
Forde, Michael M. [1 ]
Sharples, Kate [1 ]
Thetford, Adam [1 ]
Jenkins, Robert L. [1 ]
Dimitratos, Nikolaos [1 ]
Lopez-Sanchez, Jose A. [1 ]
Murphy, Damien M. [1 ]
Bethell, Donald [1 ]
Willock, David J. [1 ]
Taylor, Stuart H. [1 ]
Knight, David W. [1 ]
Kiely, Christopher J. [2 ]
Hutchings, Graham J. [1 ]
机构
[1] Cardiff Univ, Cardiff Catalysis Inst, Sch Chem, Cardiff CF10 3AT, S Glam, Wales
[2] Lehigh Univ, Ctr Adv Mat & Nanotechnol, Bethlehem, PA 18015 USA
基金
英国工程与自然科学研究理事会;
关键词
alloys; gold; heterogeneous catalysis; nanoparticles; palladium; GOLD CATALYSTS; TIO2; EPOXIDATION; MECHANISM; EPR;
D O I
10.1002/anie.201201059
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
引用
收藏
页码:5981 / 5985
页数:5
相关论文
共 50 条
  • [1] Cinnamyl alcohol oxidation using supported bimetallic Au-Pd nanoparticles: an investigation of autoxidation and catalysis
    Rucinska, Emilia
    Miedziak, Peter J.
    Pattisson, Samuel
    Brett, Gemma L.
    Iqbal, Sarwat
    Morgan, David J.
    Sankar, Meenakshisundaram
    Hutchings, Graham J.
    CATALYSIS SCIENCE & TECHNOLOGY, 2018, 8 (11) : 2987 - 2997
  • [2] Toluene total oxidation over Pd and Au nanoparticles supported on hydroxyapatite
    Chlala, Dayan
    Labaki, Madona
    Giraudon, Jean-Marc
    Gardoll, Olivier
    Denicourt-Nowicki, Audrey
    Roucoux, Alain
    Lamonier, Jean-Francois
    COMPTES RENDUS CHIMIE, 2016, 19 (04) : 525 - 537
  • [3] OXIDATION OF GLYCEROL USING TITANIA SUPPORTED Au-Pd BIMETALLIC CATALYSTS: EFFECT OF Au-Pd RATIOS ON CATALYTIC PERFORMANCE
    Nadzri, Ainol Hayah Ahmad
    Hamzah, Noraini
    Yusoff, Nik Idris Nik
    Yarmo, Mohd Ambar
    FUNCTIONAL MATERIALS LETTERS, 2011, 4 (03) : 309 - 313
  • [4] Mesoporous Cr2O3-supported Au-Pd nanoparticles: High-performance catalysts for the oxidation of toluene
    Wu, Zhixing
    Deng, Jiguang
    Xie, Shaohua
    Yang, Huanggen
    Zhao, Xingtian
    Zhang, Kunfeng
    Lin, Hongxia
    Dai, Hongxing
    Guo, Guangsheng
    MICROPOROUS AND MESOPOROUS MATERIALS, 2016, 224 : 311 - 322
  • [5] Solvent-Free Oxidation of Primary Carbon-Hydrogen Bonds in Toluene Using Au-Pd Alloy Nanoparticles
    Kesavan, Lokesh
    Tiruvalam, Ramchandra
    Ab Rahim, Mohd Hasbi
    bin Saiman, Mohd Izham
    Enache, Dan I.
    Jenkins, Robert L.
    Dimitratos, Nikolaos
    Lopez-Sanchez, Jose A.
    Taylor, Stuart H.
    Knight, David W.
    Kiely, Christopher J.
    Hutchings, Graham J.
    SCIENCE, 2011, 331 (6014) : 195 - 199
  • [6] Selective Oxidation of Saturated Hydrocarbons Using Au-Pd Alloy Nanoparticles Supported on Metal-Organic Frameworks
    Long, Jilan
    Liu, Hongli
    Wu, Shijian
    Liao, Shijun
    Li, Yingwei
    ACS CATALYSIS, 2013, 3 (04): : 647 - 654
  • [7] Highly active Au-Pd nanoparticles supported on titanate nanotubes
    Khawaji, Motaz
    Chadwick, David
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2017, 253
  • [8] Reactivity studies of Au-Pd supported nanoparticles for catalytic applications
    Lopez-Sanchez, Jose Antonio
    Dimitratos, Nikolaos
    Glanville, Neil
    Kesavan, Lokesh
    Hammond, Ceri
    Edwards, Jennifer K.
    Carley, Albert F.
    Kiely, Christopher J.
    Hutchings, Graham J.
    APPLIED CATALYSIS A-GENERAL, 2011, 391 (1-2) : 400 - 406
  • [9] Dehydrogenative Aromatization Reactions by Supported Pd or Au-Pd Alloy NanoParticles Catalysts
    Jin, Xiongjie
    Nozaki, Kyoko
    Mizuno, Noritaka
    Yamaguchi, Kazuya
    JOURNAL OF SYNTHETIC ORGANIC CHEMISTRY JAPAN, 2019, 77 (06) : 566 - 575
  • [10] Selective photocatalytic oxidation of benzene for the synthesis of phenol using engineered Au-Pd alloy nanoparticles supported on titanium dioxide
    Su, Ren
    Kesavan, Lokesh
    Jensen, Mads M.
    Tiruvalam, Ramchandra
    He, Qian
    Dimitratos, Nikolaos
    Wendt, Stefan
    Glasius, Marianne
    Kiely, Christopher J.
    Hutchings, Graham J.
    Besenbacher, Flemming
    CHEMICAL COMMUNICATIONS, 2014, 50 (84) : 12612 - 12614