The oxygen reduction activity on platinum-decorated nitrogen-doped bilayer graphene

被引：3

作者：

Wang, Ting ^{[1
]}

Liu, Jianfeng ^{[1
,2
]}

Miao, Keji ^{[1
]}

Yin, Yangyang ^{[1
]}

Ma, Junjie ^{[1
]}

Yin, Shibin ^{[3
]}

Pan, Weiguo ^{[1
,4
]}

机构：

[1] Shanghai Univ Elect Power, Coll Energy & Mech Engn, Shanghai 200120, Peoples R China

[2] Minist Educ, Guangxi Key Lab Proc Nonferrous Met & Featured Ma, Key Lab New Proc Technol Nonferrous Met & Mat, Nanning 530004, Peoples R China

[3] Guangxi Univ, Coll Chem & Chem Engn, Nanning 530004, Peoples R China

[4] Key Lab Clean Power Generat & Environm Protect Te, Shanghai 200120, Peoples R China

来源：

JOURNAL OF MATERIALS SCIENCE | 2022年 / 57卷 / 04期

关键词：

APPROXIMATION; EXCHANGE;

D O I：

10.1007/s10853-021-06677-5

中图分类号：

T [工业技术];

学科分类号：

08 ;

摘要：

Studied the oxygen reduction reaction activity of materials with different structures such as single-doped N, single-doped Pt, and double-layer graphene (BLG) co-doped with N and Pt. The BLG models under different doping conditions are established, and then oxygen molecules are adsorbed on the surface of BLG-based catalyst models. Through optimizing the structure of established models, the adsorption energy of oxygen for different models is calculated and then compares their oxygen reduction activities. Finally, it is found that the oxygen reduction activity of platinum-decorated and nitrogen-doped BLG is better than that of single doping. Meanwhile, the ORR activity of surface adsorption is also better than that of interlayer adsorption.

引用

页码：2794 / 2802

页数：9

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