Advances in rapid compression machine studies of low- and intermediate-temperature autoignition phenomena

被引:175
|
作者
Goldsborough, S. Scott [1 ]
Hochgreb, Simone [2 ]
Vanhove, Guillaume [3 ]
Wooldridge, Margaret S. [4 ]
Curran, Henry J. [5 ]
Sung, Chih-Jen [6 ]
机构
[1] Argonne Natl Lab, Ctr Transportat Res, Argonne, IL 60439 USA
[2] Univ Cambridge, Dept Engn, Cambridge CB2 1PZ, England
[3] Univ Lille, CNRS, UMR 8522, Phys Chim Proc Combust & Atmosphere PC2A, F-59000 Lille, France
[4] Univ Michigan, Dept Mech Engn, Ann Arbor, MI 48109 USA
[5] Natl Univ Ireland Galway, Combust Chem Ctr, Galway, Ireland
[6] Univ Connecticut, Dept Mech Engn, Storrs, CT 06269 USA
基金
美国国家科学基金会;
关键词
Rapid compression machine; Low temperature combustion; Chemical kinetics; Physical-chemical interactions; IGNITION DELAY TIMES; CASCADE LASER-ABSORPTION; LAMINAR FLAME SPEEDS; PREMIXED COOL FLAMES; PRESSURE SHOCK-TUBE; N-HEPTANE DROPLET; AUTO-IGNITION; CHEMICAL-KINETICS; SELF-IGNITION; PRE-IGNITION;
D O I
10.1016/j.pecs.2017.05.002
中图分类号
O414.1 [热力学];
学科分类号
摘要
Rapid compression machines (RCMs) are widely used to acquire experimental insights into fuel autoignition and pollutant formation chemistry, especially at conditions relevant to current and future combustion technologies. RCM studies emphasize important experimental regimes, characterized by low- to intermediate temperatures (600-1200 k) and moderate to high pressures (5-80 bar). At these conditions, which are directly relevant to modern combustion schemes including low temperature combustion (LTC) for internal combustion engines and dry low emissions (DLE) for gas turbine engines, combustion chemistry exhibits complex and experimentally challenging behaviors such as the chemistry attributed to cool flame behavior and the negative temperature coefficient regime. Challenges for studying this regime include that experimental observations can be more sensitive to coupled physical-chemical processes leading to phenomena such as mixed deflagrative/autoignitive combustion. Experimental strategies which leverage the strengths of RCMs have been developed in recent years to make RCMs particularly well suited for elucidating LTC and DLE chemistry, as well as convolved physical-chemical processes. Specifically, this work presents a review of experimental and computational efforts applying RCMs to study autoignition phenomena, and the insights gained through these efforts. A brief history of RCM development is presented towards the steady improvement in design, characterization, instrumentation and data analysis. Novel experimental approaches and measurement techniques, coordinated with computational methods are described which have expanded the utility of RCMs beyond empirical studies of explosion limits to increasingly detailed understanding of autoignition chemistry and the role of physical chemical interactions. Fundamental insight into the autoignition chemistry of specific fuels is described, demonstrating the extent of knowledge of low-temperature chemistry derived from RCM studies, from simple hydrocarbons to multi-component blends and full-boiling range fuels. Emerging needs and further opportunities are suggested, including investigations of under-explored fuels and the implementation of increasingly higher fidelity diagnostics. (C) 2017 Elsevier Ltd. All rights reserved.
引用
收藏
页码:1 / 78
页数:78
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