Characteristics of an Integrated Micro Packed Bed Reactor-Heat Exchanger for methanol synthesis from syngas

被引：57

作者：

Bakhtiary-Davijany, Hamidreza ^{[1
]}

Hayer, Fatemeh ^{[1
]}

Phan, Xuyen Kim ^{[1
]}

Myrstad, Rune ^{[2
]}

Venvik, Hilde J. ^{[1
]}

Pfeifer, Peter ^{[3
]}

Holmen, Anders ^{[1
]}

机构：

[1] Norwegian Univ Sci & Technol NTNU, Dept Chem Engn, NO-7491 Trondheim, Norway

[2] SINTEF Mat & Chem, NO-7465 Trondheim, Norway

[3] Karlsruhe Inst Technol KIT, Inst Micro Proc Engn IMVT, DE-76344 Eggenstein Leopoldshafen, Germany

来源：

CHEMICAL ENGINEERING JOURNAL | 2011年 / 167卷 / 2-3期

关键词：

Micro Packed Bed Reactor; Off shore gas conversion; Methanol; Microchannel; Isothermal operation; Pressure drop; Fluid flow; FISCHER-TROPSCH SYNTHESIS; LIMITATIONS; MICROCHANNEL;

D O I：

10.1016/j.cej.2010.08.074

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

The main characteristics of a multi-slit Integrated Micro Packed Bed Reactor-Heat Exchanger (IMPBRHE) for compact synthesis of methanol from syngas over a Cu/ZnO/Al2O3 catalyst under industrial operating conditions (80 bar and 523 K) were investigated. The reaction experiments show that near equilibrium conversion per pass is achievable at low contact times (about 470 ms g/ml). The experiments show superior heat removal capability from the catalytic slits through isothermal conditions. Pressure drop measurements in agreement with calculation by Ergun equation indicate an isobaric reaction media in the slits. The IMPBRHE shows promising features for further research on process intensification and miniaturization. (C) 2010 Elsevier BM. All rights reserved.

引用

页码：496 / 503

页数：8

共 50 条

[1] Characteristics of integrated micro packed bed reactor-heat exchanger configurations in the direct synthesis of dimethyl ether
Hayer, Fatemeh
Bakhtiary-Davijany, Hamidreza
Myrstad, Rune
Holmen, Anders
Pfeifer, Peter
Venvik, Hilde J.
CHEMICAL ENGINEERING AND PROCESSING-PROCESS INTENSIFICATION, 2013, 70 : 77 - 85
[2] Modeling and Simulation of an Integrated Micro Packed Bed Reactor-Heat Exchanger Configuration for Direct Dimethyl Ether Synthesis
Fatemeh Hayer
Hamidreza Bakhtiary-Davijany
Rune Myrstad
Anders Holmen
Peter Pfeifer
Hilde J. Venvik
Topics in Catalysis, 2011, 54
[3] Modeling and Simulation of an Integrated Micro Packed Bed Reactor-Heat Exchanger Configuration for Direct Dimethyl Ether Synthesis
Hayer, Fatemeh
Bakhtiary-Davijany, Hamidreza
Myrstad, Rune
Holmen, Anders
Pfeifer, Peter
Venvik, Hilde J.
TOPICS IN CATALYSIS, 2011, 54 (13-15) : 817 - 827
[4] NUMERICAL INVESTIGATION OF THERMOCHEMICAL ENERGY EXTRACTION IN A MOVING PACKED BED OXIDATION REACTOR-HEAT EXCHANGER
Mishra, Ashreet
Korba, David
Li, Like
PROCEEDINGS OF ASME 2023 17TH INTERNATIONAL CONFERENCE ON ENERGY SUSTAINABILITY, ES2023, 2023,
[5] Modelling and simulation of a single slit micro packed bed reactor for methanol synthesis
Bakhtiary-Davijany, Hamidreza
Hayer, Fatemeh
Phan, Xuyen Kim
Myrstad, Rune
Venvik, Hilde J.
Pfeifer, Peter
Holmen, Anders
CATALYSIS TODAY, 2020, 343 (343) : 226 - 233
[6] Heat transfer characteristics analysis and optimization of the Micro Packed Bed Bionic Reactor
Liu, Wei-liao
Li, Xi
Cheng, You-wei
Wang, Li-jun
CHEMICAL ENGINEERING AND PROCESSING-PROCESS INTENSIFICATION, 2019, 144
[7] Radial Reactor-Heat Exchanger for Natural Gas Combustion in a Structured Porous Metal Catalyst Bed
V. A. Kirillov
N. A. Kuzin
V. A. Kuz’min
V. B. Skomorokhov
A. B. Shigarov
Theoretical Foundations of Chemical Engineering, 2005, 39 : 407 - 414
[8] Radial reactor-heat exchanger for natural gas combustion in a structured porous metal catalyst bed
Kirillov, VA
Kuzin, NA
Kuz'min, VA
Skomorokhov, VB
Shigarov, AB
THEORETICAL FOUNDATIONS OF CHEMICAL ENGINEERING, 2005, 39 (04) : 407 - 414
[9] A micro packed-bed reactor for chemical synthesis
Losey, MW
Schmidt, MA
Jensen, KF
MICROREACTION TECHNOLOGY: INDUSTRIAL PROSPECTS, 2000, : 277 - 286
[10] Methanol synthesis in a fluidized-bed reactor coupled with an external heat exchanger - The effect of feedback deformation
Tabis, B
CHEMICAL ENGINEERING JOURNAL, 2001, 83 (03) : 191 - 200

← 1 2 3 4 5 →