The influence of residential wood combustion on the concentrations of PM2.5 in four Nordic cities

被引:39
|
作者
Kukkonen, Jaakko [1 ]
Lopez-Aparicio, Susana [2 ]
Segersson, David [3 ]
Geels, Camilla [4 ]
Kangas, Leena [1 ]
Kauhaniemi, Mari [1 ]
Maragkidou, Androniki [1 ]
Jensen, Anne [4 ]
Assmuth, Timo [5 ]
Karppinen, Ari [1 ]
Sofiev, Mikhail [1 ]
Hellen, Heidi [1 ]
Riikonen, Kari [1 ]
Nikmo, Juha [1 ]
Kousa, Anu [6 ]
Niemi, Jarkko, V [6 ]
Karvosenoja, Niko [5 ]
Santos, Gabriela Sousa [2 ]
Sundvor, Ingrid [7 ]
Im, Ulas [4 ]
Christensen, Jesper Heile [4 ]
Nielsen, Ole-Kenneth [4 ]
Plejdrup, Marlene [4 ]
Nojgaard, Jacob Kleno [4 ]
Omstedt, Gunnar [3 ]
Andersson, Camilla [3 ]
Forsberg, Bertil [8 ]
Brandt, Jorgen [4 ]
机构
[1] Finnish Meteorol Inst, Erik Palmenin Aukio 1,POB 503, FIN-00101 Helsinki, Finland
[2] Norwegian Inst Air Res, Inst Veien 18,POB 100, N-2027 Kjeller, Norway
[3] Swedish Meteorol & Hydrol Inst, S-60176 Norrkoping, Sweden
[4] Aarhus Univ, Dept Environm Sci Atmospher Modeling, Frederiksborgvej 399, DK-4000 Roskilde, Denmark
[5] Finnish Environm Inst, Latokartanonkaari 11, Helsinki 00790, Finland
[6] Helsinki Reg Environm Serv Author, Ilmalantori 1, Helsinki 00240, Finland
[7] Inst Transport Econ, Gaustadalleen 21, N-0349 Oslo, Norway
[8] Umea Univ, Dept Publ Hlth & Clin Med, S-90187 Umea, Sweden
基金
芬兰科学院;
关键词
PARTICULATE AIR-POLLUTION; HELSINKI METROPOLITAN-AREA; DISPERSION MODELING SYSTEM; CARBONACEOUS AEROSOL; SOURCE APPORTIONMENT; ROAD DUST; HIGH-RESOLUTION; NORTH-AMERICA; EMISSIONS; EUROPE;
D O I
10.5194/acp-20-4333-2020
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Residential wood combustion (RWC) is an important contributor to air quality in numerous regions worldwide. This study is the first extensive evaluation of the influence of RWC on ambient air quality in several Nordic cities. We have analysed the emissions and concentrations of PM2.5 in cities within four Nordic countries: in the metropolitan areas of Copenhagen, Oslo, and Helsinki and in the city of Umea. We have evaluated the emissions for the relevant urban source categories and modelled atmospheric dispersion on regional and urban scales. The emission inventories for RWC were based on local surveys, the amount of wood combusted, combustion technologies and other relevant factors. The accuracy of the predicted concentrations was evaluated based on urban concentration measurements. The predicted annual average concentrations ranged spatially from 4 to 7 mu g m(-3) (2011), from 6 to 10 mu g m(-3) (2013), from 4 to more than 13 mu g m(-3) (2013) and from 9 to more than 13 mu g m(-3) (2014), in Umea, Helsinki, Oslo and Copenhagen, respectively. The higher concentrations in Copenhagen were mainly caused by the relatively high regionally and continentally transported background contributions. The annual av-erage fractions of PM2.5 concentrations attributed to RWC within the considered urban regions ranged spatially from 0% to 15 %, from 0% to 20 %, from 8% to 22% and from 0% to 60% in Helsinki, Copenhagen, Umea and Oslo, respectively. In particular, the contributions of RWC in central Oslo were larger than 40% as annual averages. In Oslo, wood combustion was used mainly for the heating of larger blocks of flats. In contrast, in Helsinki, RWC was solely used in smaller detached houses. In Copenhagen and Helsinki, the highest fractions occurred outside the city centre in the suburban areas. In Umea, the highest fractions occurred both in the city centre and its surroundings.
引用
收藏
页码:4333 / 4365
页数:33
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