Preparation and performance of a biological dust suppressant based on the synergistic effect of enzyme-induced carbonate precipitation and surfactant

被引:10
|
作者
Wu, Mingyue [1 ]
Hu, Xiangming [1 ,2 ,3 ]
Zhang, Qian [1 ]
Zhao, Yanyun [1 ]
Cheng, Weimin [1 ]
Xue, Di [1 ]
机构
[1] Shandong Univ Sci & Technol, Coll Safety & Environm Engn, Qingdao 266590, Shandong, Peoples R China
[2] Shandong Univ Sci & Technol, State Key Lab Min Lab Disaster Prevent & Control, Qingdao 266590, Shandong, Peoples R China
[3] Shandong Univ Sci & Technol, Minist Sci & Technol, Qingdao 266590, Shandong, Peoples R China
基金
中国国家自然科学基金; 国家重点研发计划;
关键词
Surfactant; Enzyme-induced carbonate precipitation; Urease activity; Wind resistance; Molecular simulation; Dust consolidation; MOLECULAR-DYNAMICS; NONIONIC SURFACTANTS; COAL; WETTABILITY; FACE; CFD;
D O I
10.1007/s11356-021-16307-x
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
To control the dust pollution caused by open-pit coal mining and reduce or avoid the secondary hazards of existing dust suppressants to the environment, a biological dust suppressant was prepared through the synergistic effect of a surfactant and an enzyme-induced carbonate precipitation. The optimal ratio of biological dust suppressant was determined, and the dust suppressive effect and dust consolidation mechanism of the biological dust suppressant were investigated. The results showed that the optimal biological dust suppressant had an alkyl polyglycoside (APG) concentration of 0.3 wt.%, a urea-CaCl2 concentration of 0.6 mol/L, and a urease to urea-CaCl2 volume ratio of 1:3. The wind erosion resistance of coal dust treated with this dust suppressant was enhanced by 86.69%. The adsorption of the biological dust suppressant by coal dust was mainly due to the electrostatic interaction between the surfactant and coal dust. The mineralization product of the dust suppressant was calcite-type CaCO3, which consolidated coal dust due to the formation of intermolecular hydrogen bonds between CaCO3 and coal dust.
引用
收藏
页码:8423 / 8437
页数:15
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