Construction of Hexagonal Prisms of Variable Size via Coordination-Driven Multicomponent Self-Assembly

被引：39
|
作者：
Zhao, Zhigang [1 ]
Zheng, Yao-Rong [1 ]
Wang, Ming [1 ]
Pollock, J. Bryant [1 ]
Stang, Peter J. [1 ]
机构：
[1] Univ Utah, Dept Chem, Salt Lake City, UT 84112 USA
来源：
INORGANIC CHEMISTRY | 2010年 / 49卷 / 19期
关键词：
DYNAMIC COMBINATORIAL CHEMISTRY; CAGE-LIKE COMPLEX; SUPRAMOLECULAR CHEMISTRY; METALLACYCLIC POLYGONS; MOLECULAR RECOGNITION; PD(II)-LINKED CAGES; TEMPLATE SYNTHESIS; TRANSITION-METALS; RATIONAL DESIGN; BORROMEAN RINGS;
D O I：
10.1021/ic1014219
中图分类号：
O61 [无机化学];
学科分类号：
070301 ; 081704 ;
摘要：
The coordination-driven self-assembly of supramolecular hexagonal prisms has been achieved upon mixing a hexakis[4-(4-pyridyl)phenyl]benzene donor ligand and carboxylate donor ligands such as sodium terephthalate, sodium (1,1'-biphenyl)-4,4'-dicarboxylate, sodium 4,4'-(diazene-1,2-diyl)dibenzoate, and 4,4'-dipyridyl with cis-Pt(PEt3)(2)(OTf)(2) in a 1:3:6 ratio. Four assembled hexagonal prisms have been characterized by P-31 and H-1 NMR multinuclear spectroscopy as well as electrospray ionization mass spectrometry. Molecular force-field simulations provide the possible conformation and size of each structure.
引用
收藏
页码：8653 / 8655
页数：3
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