Growth and characterization of Ce-doped Ca3(BO3)2 crystals for neutron scintillator

被引:19
|
作者
Fujimoto, Yutaka [1 ,2 ]
Yanagida, Takayuki [1 ]
Tanaka, Hidehiko [1 ]
Yokota, Yuui [1 ]
Kawaguti, Noriaki [4 ]
Fukuda, Kentaro [1 ,4 ]
Totsuka, Daisuke [5 ]
Watanabe, Kenichi [6 ]
Yamazaki, Atsushi [6 ]
Yoshikawa, Akira [1 ,3 ]
机构
[1] Tohoku Univ, IMRAM, Aoba Ku, Sendai, Miyagi 9808577, Japan
[2] JSPS, Chiyoda Ku, Tokyo 1028472, Japan
[3] Tohoku Univ, NICHe, Aoba Ku, Sendai, Miyagi 9808579, Japan
[4] TOKUYAMA Corp, Shibuya Ku, Tokyo 1508383, Japan
[5] NIHON KESSHO KOGAKU CO LTD, Tatebayashi Gunma, Japan
[6] Nagoya Univ, Chikusa Ku, Nagoya, Aichi 4648603, Japan
关键词
Czochralski method; Borates; Scintillator materials; Scintillators; SINGLE-CRYSTALS; LAB3O6; PURE;
D O I
10.1016/j.jcrysgro.2010.10.189
中图分类号
O7 [晶体学];
学科分类号
0702 ; 070205 ; 0703 ; 080501 ;
摘要
Single crystals of undoped and Ce3+-doped Ca-3(BO3)(2) (CBO) are grown by the Czochralski (CZ) method with an RF heating system. Undoped CBO crystal has high transmittance in the 190-900 nm wavelength range, while the absorption bands were observed around 275 and 350 nm due to the transition from the 4f ground state levels of F-2(5/2) and F-2(7/2) to Ce3+ 5d excited state in Ce3+-doped one. The photoluminescence spectrum of Ce3+-doped CBO crystal showed strong emission band around 400 nm under both 275 and 350 nm excitation due to the 5d-4f transition of Ce3+. In the measurement of pulse height spectra under Am-241 5.5 MeV alpha-ray excitation, Ce3+-doped CBO showed higher energy resolution compared with that of crystal grown by the micro-pulling down (mu-PD) method. (C) 2010 Elsevier B.V. All rights reserved.
引用
收藏
页码:784 / 787
页数:4
相关论文
共 50 条
  • [1] Growth of birefringent Ca3(BO3)2 crystals by the Czochralski method
    Zhang, SY
    Wu, X
    Song, YT
    Ni, DQ
    Hu, BQ
    Zhou, T
    JOURNAL OF CRYSTAL GROWTH, 2003, 252 (1-3) : 246 - 250
  • [2] Unravelling the effect of interstitial oxygen on the photoluminescence of Ce3+-doped Ca2BO3Cl and Ca3(BO3)2
    Ablat, Aynigar
    Yin, Min
    Zhou, Shihang
    Sidike, Aierken
    JOURNAL OF LUMINESCENCE, 2025, 279
  • [3] Optical and scintillation properties of Pr3+-doped Ca3(BO3)2 single crystals
    Fujimoto, Y.
    Yanagida, T.
    Yokota, Y.
    Kawaguchi, N.
    Fukuda, K.
    Totsuka, D.
    Watanabe, K.
    Yamazaki, A.
    Chani, V.
    Yoshikawa, A.
    PHYSICA STATUS SOLIDI B-BASIC SOLID STATE PHYSICS, 2011, 248 (02): : 444 - 447
  • [4] Scintillation characteristics of Tm3+ in Ca3(BO3)2 crystals
    Fujimoto, Yutaka
    Yanagida, Takayuki
    Yokota, Yuui
    Kawaguchi, Noriaki
    Fukuda, Kentaro
    Totsuka, Daisuke
    Watanabe, Kenichi
    Yamazaki, Atsushi
    Yoshikawa, Akira
    RADIATION MEASUREMENTS, 2011, 46 (12) : 1506 - 1508
  • [5] Bulk Growth, Thermal, and Polarized Spectral Characters of Nd3+-Doped Ca3(BO3)2 Single Crystals
    Yu, Pingzhang
    Qi, Hongwei
    Liu, Yanqing
    Yu, Fapeng
    Wang, Zhengping
    Dang, Yangyang
    CRYSTAL RESEARCH AND TECHNOLOGY, 2025, 60 (02)
  • [6] Optical properties of Er3+ doped Ca3 (BO3)2 crystal
    Lu, Xiuai
    You, Zhenyu
    Li, Jianfu
    Zhu, Zhaojie
    Jia, Guohua
    Wu, Baichang
    Tu, Chaoyang
    JOURNAL OF APPLIED PHYSICS, 2006, 100 (03)
  • [7] Crystal growth and luminescent properties of the Ce-doped Li6Lu(BO3)3
    Yang, F.
    Pan, S. K.
    Ding, D. Z.
    Chen, X. F.
    Feng, H.
    Ren, G. H.
    JOURNAL OF CRYSTAL GROWTH, 2010, 312 (16-17) : 2411 - 2414
  • [9] Growth and properties of pure and rare earth-doped Ca3 (BO3)2 single crystal
    Lu, X
    You, ZY
    Li, JF
    Zhu, ZJ
    Jia, GH
    Wang, Y
    Wu, BC
    Tu, CY
    JOURNAL OF CRYSTAL GROWTH, 2005, 281 (2-4) : 416 - 425
  • [10] Transparent Microcomposite Films Based on a Ce-Doped Li6Gd(BO3)3 Scintillator for Radiation Detection
    Zhou, Xunsheng
    Wang, Cai Lin
    Wang, Yinzhen
    ACS OMEGA, 2022, 7 (35): : 31567 - 31576