Technical challenges in tackling regulatory concerns for urban atmospheric nanoparticles

被引:39
|
作者
Kumar, Prashant [1 ,2 ]
Robins, Alan [2 ]
Vardoulakis, Sotiris [3 ]
Quincey, Paul [4 ]
机构
[1] Univ Surrey, FEPS, Div Civil Chem & Environm Engn, Guildford GU2 7XH, Surrey, England
[2] Univ Surrey, FEPS, Environm Flow EnFlo Res Ctr, Guildford GU2 7XH, Surrey, England
[3] Hlth Protect Agcy, Ctr Radiat Chem & Environm Hazards, Chilton OX11 0RQ, Oxon, England
[4] Natl Phys Lab, Analyt Sci Div, Teddington TW11 0LW, Middx, England
基金
英国工程与自然科学研究理事会;
关键词
Airborne and manufactured nanoparticles; Particle number concentrations; Size distributions; Street canyons; Ultrafine particles; Vehicle emissions; AEROSOL-SIZE DISTRIBUTIONS; PARTICLE NUMBER; AIR-QUALITY; ULTRAFINE PARTICLES; EMISSIONS; BIODIESEL; STREET; DIESEL; DISPERSION; FINE;
D O I
10.1016/j.partic.2011.06.002
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Recent Euro 5 and Euro 6 vehicle emission standards are the first ever initiative to control particles on a number basis at the source. Related standards are also desirable for ambient nanoparticles (taken in this article to be those below 300 nm) to protect against possible adverse effects on public health and the environment. However, there are a number of technical challenges that need to be tackled before developing a regulatory framework for atmospheric nanoparticles. Some of the challenges derive from a lack of standardisation of the key measurement parameters, including sampling, necessary for robust evaluation of particle number concentrations, especially in the context of insufficient knowledge of the physicochemical characteristics of emerging sources (i.e. bio-fuel derived and manufactured nanoparticles). Ideally, ambient concentrations of primary particles could be linked to primary particle emissions by use of nanoparticle dispersion models, and secondary nanoparticles using photochemical modeling tools. The limitations in these areas are discussed. Although there is inadequate information on the exact biological mechanism through which these particles cause harm, it is argued that this should not in itself delay the introduction of regulation. This article reviews the missing links between the existing knowledge of nanoparticle number concentrations and the advances required to tackle the technical challenges implied in developing regulations. (C) 2011 Chinese Society of Particuology and Institute of Process Engineering, Chinese Academy of Sciences. Published by Elsevier B.V. All rights reserved.
引用
收藏
页码:566 / 571
页数:6
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