Nonequilibrium dynamics of mixtures of active and passive colloidal particles

被引:62
|
作者
Wittkowski, Raphael [1 ,2 ]
Stenhammar, Joakim [3 ]
Cates, Michael E. [4 ]
机构
[1] Westfalische Wilhelms Univ Munster, Inst Theoret Phys, D-48149 Munster, Germany
[2] Westfalische Wilhelms Univ Munster, Ctr Nonlinear Sci CeNoS, D-48149 Munster, Germany
[3] Lund Univ, Div Phys Chem, SE-22100 Lund, Sweden
[4] Univ Cambridge, Ctr Math Sci, DAMTP, Cambridge CB3 0WA, England
来源
NEW JOURNAL OF PHYSICS | 2017年 / 19卷
基金
瑞典研究理事会;
关键词
active colloidal particles; active-passive mixtures; motility-induced instability; mesoscopic field theory particle-resolved simulations;
D O I
10.1088/1367-2630/aa8195
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We develop a mesoscopic field theory for the collective nonequilibrium dynamics of multicomponent mixtures of interacting active (i.e., motile) and passive (i.e., nonmotile) colloidal particles with isometric shape in two spatial dimensions. By a stability analysis of the field theory, we obtain equations for the spinodal that describes the onset of a motility-induced instability leading to cluster formation in such mixtures. The prediction for the spinodal is found to be in good agreement with particle-resolved computer simulations. Furthermore, we show that in active-passive mixtures the spinodal instability can be of two different types. One type is associated with a stationary bifurcation and occurs also in one-component active systems, whereas the other type is associated with a Hopf bifurcation and can occur only in active-passive mixtures. Remarkably, the Hopf bifurcation leads to moving clusters. This explains recent results from simulations of active-passive particle mixtures, where moving clusters and interfaces that are not seen in the corresponding one-component systems have been observed.
引用
收藏
页数:16
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