Interaction of the charged deuterium cluster D3+ with femtosecond laser pulses

被引:14
|
作者
Isla, M. [1 ]
Alonso, J. A.
机构
[1] Univ Valladolid, Dept Fis Teor Atom & Opt, E-47005 Valladolid, Spain
[2] DIPC, E-20018 San Sebastian, Spain
来源
JOURNAL OF PHYSICAL CHEMISTRY C | 2007年 / 111卷 / 48期
关键词
D O I
10.1021/jp070717+
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
A computational study of the dynamics of the charged deuterium trimer D-3(+) under irradiation by feratosecond laser pulses is presented. The computer simulations are carried out in the frame of a nonadiabatic, nonlinearized model of the coupled evolution of electrons and ions based on the time dependent density functional theory (TDDFT). Several laser field parameters such as intensity, frequency, and polarization have been varied, and their effects on the excitation of the cluster have been analyzed. A proper choice of the laser parameters can be used to lead the trimer across one of the several excitation output channels, from a perturbative regime at low intensities to a nonlinear domain with the occurrence of Coulomb explosion at high intensities.
引用
收藏
页码:17765 / 17772
页数:8
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