VOC concentrations measured in personal samples and residential indoor, outdoor and workplace microenvironments in EXPOLIS-Helsinki, Finland

被引:163
|
作者
Edwards, RD
Jurvelin, J
Saarela, K
Jantunen, M
机构
[1] Finnish Natl Inst Publ Hlth, KTL, Dept Environm Hyg, FIN-70701 Kuopio, Finland
[2] Univ Calif Berkeley, Sch Publ Hlth, Berkeley, CA 94720 USA
[3] Jyvaskula Polytech, Sch Engn & Technol, Jyvaskyla, Finland
[4] VTT, Chem Technol, Espoo, Finland
[5] EC, JRC, Inst Environm, Ispra, Italy
基金
芬兰科学院;
关键词
personal exposure; indoor concentrations; volatile organic compounds; street traffic; environmental tobacco smoke;
D O I
10.1016/S1352-2310(01)00230-8
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Thirty target volatile organic compounds (VOC) were analyzed in personal 48-h exposure samples and residential indoor, residential outdoor and workplace indoor microenvironment samples as a component of EXPOLIS-Helsinki, Finland. Geometric mean residential indoor concentrations were higher than geometric mean residential outdoor concentrations for all target compounds except hexane, which was detected in 40% of residential outdoor samples and 11% of residential indoor samples, respectively. Geometric mean residential indoor concentrations were significantly higher than personal exposure concentrations, which in turn were significantly higher than workplace concentrations for compounds that had strong residential indoor sources (d-limonene, alpha pinene, 3-carene, hexanal, 2-methyl-1-propanol and 1-butanol). 40% of participants in EXPOLIS- Helsinki reported personal exposure to environmental tobacco smoke (ETS). Participants in Helsinki that were exposed to ETS at any time during the 48-h sampling period had significantly higher personal exposures to benzene, toluene, styrene, m,p-xylene, o-xylene. ethylbenzene and trimethylbenzene. Geometric mean ETS-free workplace concentrations were higher than ETS-free personal exposure concentrations for styrene, hexane and cyclohexane. Geometric mean personal exposures of participants not exposed to ETS were approximately equivalent to time weighted ETS-free indoor and workplace concentrations, except for octanal and compounds associated with traffic, which showed higher geometric mean personal exposure concentrations than any microenvironment (o-xylene, ethylbenzene, benzene, undecane, nonane, decane, m,p-xylene, and trimethylbenzene). Considerable differences in personal exposure concentrations and residential levels of compounds with mainly indoor sources suggested differences in product types or the frequency of product use between Helsinki, Germany and the United States. (C) 2001 Elsevier Science Ltd. All rights reserved.
引用
收藏
页码:4531 / 4543
页数:13
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共 32 条
  • [1] VOC source identification from personal and residential indoor, outdoor and workplace microenvironment samples in EXPOLIS-Helsinki, Finland
    Edwards, RD
    Jurvelin, J
    Koistinen, K
    Saarela, K
    Jantunen, M
    [J]. ATMOSPHERIC ENVIRONMENT, 2001, 35 (28) : 4829 - 4841
  • [2] Sources of fine particulate matter in personal exposures and residential indoor, residential outdoor and workplace microenvironments in the Helsinki phase of the EXPOLIS study
    Koistinen, KJ
    Edwards, RD
    Mathys, P
    Ruuskanen, J
    Künzli, N
    Jantunen, MJ
    [J]. SCANDINAVIAN JOURNAL OF WORK ENVIRONMENT & HEALTH, 2004, 30 : 36 - 46
  • [3] Personal exposures to NO2 in the EXPOLIS-study:: relation to residential indoor, outdoor and workplace concentrations in Basel, Helsinki and Prague
    Kousa, A
    Monn, C
    Rotko, T
    Alm, S
    Oglesby, L
    Jantunen, MJ
    [J]. ATMOSPHERIC ENVIRONMENT, 2001, 35 (20) : 3405 - 3412
  • [4] Personal PM2.5 exposures residential and workplace indoor and residential outdoor concentrations:: Comparison of seven European cities in the Expolis study
    Jantunen, M
    Nieuwenhuijsen, M
    Künzli, N
    Zmirou, D
    Sram, R
    Katsouyanni, K
    Maroni, M
    [J]. EPIDEMIOLOGY, 2002, 13 (04) : S238 - S239
  • [5] Personal exposures to VOC in the upper end of the distribution -: relationships to indoor, outdoor and workplace concentrations
    Edwards, RD
    Schweizer, C
    Jantunen, M
    Lai, HK
    Bayer-Oglesby, L
    Katsouyanni, K
    Nieuwenhuijsen, M
    Saarela, K
    Sram, R
    Künzli, N
    [J]. ATMOSPHERIC ENVIRONMENT, 2005, 39 (12) : 2299 - 2307
  • [6] Residential indoor, outdoor, and workplace concentrations of carbonyl compounds: Relationships with personal exposure concentrations and correlation with sources
    Jurvelin, JA
    Edwards, RD
    Vartiainen, M
    Pasanen, P
    Jantunen, MJ
    [J]. JOURNAL OF THE AIR & WASTE MANAGEMENT ASSOCIATION, 2003, 53 (05): : 560 - 573
  • [7] Evaluation of VOC concentrations in indoor and outdoor microenvironments at near-road schools
    Raysoni, Amit U.
    Stock, Thomas H.
    Sarnat, Jeremy A.
    Chavez, Mayra C.
    Sarnat, Stefanie Ebelt
    Montoya, Teresa
    Holguin, Fernando
    Li, Wen-Whai
    [J]. ENVIRONMENTAL POLLUTION, 2017, 231 : 681 - 693
  • [8] CHARACTERISTICS OF ALDEHYDES - CONCENTRATIONS, SOURCES, AND EXPOSURES FOR INDOOR AND OUTDOOR RESIDENTIAL MICROENVIRONMENTS
    ZHANG, JF
    HE, QC
    LIOY, PJ
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1994, 28 (01) : 146 - 152
  • [9] Determinants of personal, indoor and outdoor VOC concentrations: An analysis of the RIOPA data
    Su, Feng-Chiao
    Mukherjee, Bhramar
    Batterman, Stuart
    [J]. ENVIRONMENTAL RESEARCH, 2013, 126 : 192 - 203
  • [10] Characteristics of carbonyls: Concentrations and source strengths for indoor and outdoor residential microenvironments in China
    Wang, B.
    Lee, S. C.
    Ho, K. F.
    [J]. ATMOSPHERIC ENVIRONMENT, 2007, 41 (13) : 2851 - 2861