We have analysed in detail four selected episodes involving substantially high concentrations of PM(10) that occurred in Oslo on 4-10 January 2003, in Helsinki on 3-14 April 2002, in London on 18-27 February 2003 and in Milan on 14-19 December 1998. We have also utilised a more extensive dataset containing relevant information regarding 21 episodes from seven cities in six countries. The four episodes analysed in detail were recently occurring cases that were at least partly caused by various local emission sources. In particular, we have addressed the evolution of the measured concentrations in terms of the measured, meteorologically pre-processed and predicted (using numerical weather prediction models and a meso-scale meteorological model) meteorological variables. All the four episodes addressed were associated with areas of high pressure (Oslo, Helsinki and London) or a high-pressure ridge (Milan). The best meteorological prediction variables were found to be the temporal evolution of the temperature inversions and atmospheric stability and, in some of the cases, wind speed. Strong ground-based or slightly elevated temperature inversions prevailed in the course of the episodes in Oslo, Helsinki and Milan, and there was a slight ground-based inversion also in London; their occurrence coinciding with the highest PM(10) concentrations. The same result was also obtained by considering an additional set of seven PM(10) episodes from the larger dataset. The inversions in Oslo and Milan were mainly caused by the advection of warmer air above a relatively colder surface, and that in Helsinki by radiation cooling of snow-covered ground. It was also found that a low wind speed is not necessarily a good indicator of episodes; this is the case, e.g., in the Po valley, due to the frequently occurring calm and low wind speed conditions there. (c) 2005 Elsevier Ltd. All rights reserved.
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Helsinki Metropolitan Area Council YTV, Environm Off, FI-00521 Helsinki, FinlandHelsinki Metropolitan Area Council YTV, Environm Off, FI-00521 Helsinki, Finland
Aarnio, Paivi
Martikainen, Jyrki
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Univ Helsinki, Dept Phys Sci, FI-00014 Helsinki, FinlandHelsinki Metropolitan Area Council YTV, Environm Off, FI-00521 Helsinki, Finland
Martikainen, Jyrki
Hussein, Tareq
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Univ Helsinki, Dept Phys Sci, FI-00014 Helsinki, FinlandHelsinki Metropolitan Area Council YTV, Environm Off, FI-00521 Helsinki, Finland
Hussein, Tareq
Valkama, Ilkka
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FMI, FI-00101 Helsinki, FinlandHelsinki Metropolitan Area Council YTV, Environm Off, FI-00521 Helsinki, Finland
Valkama, Ilkka
Vehkamaki, Hanna
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Univ Helsinki, Dept Phys Sci, FI-00014 Helsinki, FinlandHelsinki Metropolitan Area Council YTV, Environm Off, FI-00521 Helsinki, Finland
Vehkamaki, Hanna
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Sogacheva, Larisa
Harkonen, Jari
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FMI, FI-00101 Helsinki, FinlandHelsinki Metropolitan Area Council YTV, Environm Off, FI-00521 Helsinki, Finland
Harkonen, Jari
Karppinen, Ari
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FMI, FI-00101 Helsinki, FinlandHelsinki Metropolitan Area Council YTV, Environm Off, FI-00521 Helsinki, Finland
Karppinen, Ari
Koskentalo, Tarja
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Helsinki Metropolitan Area Council YTV, Environm Off, FI-00521 Helsinki, FinlandHelsinki Metropolitan Area Council YTV, Environm Off, FI-00521 Helsinki, Finland
Koskentalo, Tarja
Kukkonen, Jaakko
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机构:Helsinki Metropolitan Area Council YTV, Environm Off, FI-00521 Helsinki, Finland
Kukkonen, Jaakko
Kulmala, Markku
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Univ Helsinki, Dept Phys Sci, FI-00014 Helsinki, FinlandHelsinki Metropolitan Area Council YTV, Environm Off, FI-00521 Helsinki, Finland
机构:
Warsaw University of Technology,Department of Environmental Engineering, Faculty of Building Services, Hydro and Environmental EngineeringWarsaw University of Technology,Department of Environmental Engineering, Faculty of Building Services, Hydro and Environmental Engineering