Recent Advances in Blue Perovskite Quantum Dots for Light-Emitting Diodes

被引:54
|
作者
He, Haiyang [1 ]
Mei, Shiliang [2 ]
Wen, Zhuoqi [3 ]
Yang, Dan [1 ]
Yang, Bobo [3 ]
Zhang, Wanlu [1 ]
Xie, Fengxian [1 ]
Xing, Guichuan [2 ]
Guo, Ruiqian [1 ,3 ,4 ,5 ]
机构
[1] Fudan Univ, Sch Informat Sci & Technol, Inst Elect Light Sources, Shanghai 200433, Peoples R China
[2] Univ Macau, Inst Appl Phys & Mat Engn, Ave Univ, Taipa 999078, Macau, Peoples R China
[3] Fudan Univ, Acad Engn & Technol, Inst Future Lighting, Shanghai 200433, Peoples R China
[4] Zhongshan Fudan Joint Innovat Ctr, Zhongshan 528437, Peoples R China
[5] Fudan Univ, Yiwu Res Inst, Chengbei Rd, Yiwu City 322000, Zhejiang, Peoples R China
基金
中国国家自然科学基金;
关键词
blue emission; light-emitting diodes; metal halide perovskite; quantum dots; ROOM-TEMPERATURE SYNTHESIS; MIXED-HALIDE PEROVSKITES; SELF-TRAPPED EXCITONS; LEAD-FREE; EFFICIENT BLUE; CSPBX3; X; COLLOIDAL NANOCRYSTALS; PHASE SEGREGATION; BR; PHOTOLUMINESCENCE;
D O I
10.1002/smll.202103527
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Metal halide perovskite nanostructures have sparked intense research interest due to their excellent optical properties. In recent years, although the green and red perovskite light-emitting diodes (PeLEDs) have achieved a significant breakthrough with the external quantum efficiency exceeding 20%, the blue PeLEDs still suffer from inferior performance. Previous reviews about blue PeLEDs focus more on 2D/quasi-2D or 3D perovskite materials. To develop more stable and efficient blue PeLEDs, a systematic review of blue perovskite quantum dots (PQDs) is urgently demanded to clarify how PQDs evolve. In this review, the recent advances in blue PQDs involving mixed-halide, quantum-confined all-bromide, metal-doped and lead-free PQDs as well as their applications in PeLEDs are highlighted. Although several excellent PeLEDs based on these PQDs have been demonstrated, there are still many problems to be solved. A deep insight into the advantages and disadvantages of these four types of blue-emitting PQDs is provided. Then, their respective potential and issues for blue PeLEDs have been discussed. Finally, the challenges and outlook for efficient and stable blue PeLEDs based on PQDs are addressed.
引用
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页数:29
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