Resolution Enhancement in Wide-Field IR Imaging and Time-Domain Spectroscopy Using Dielectric Microspheres

被引:9
|
作者
Edun, Dean N. [1 ]
Nelmark, Claire E. [1 ]
Serrano, Arnaldo L. [1 ]
机构
[1] Univ Notre Dame, Dept Chem & Biochem, Indianapolis, IN 46544 USA
来源
JOURNAL OF PHYSICAL CHEMISTRY A | 2020年 / 124卷 / 27期
关键词
INFRARED-SPECTROSCOPY; MICROSCOPY;
D O I
10.1021/acs.jpca.0c02418
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Wide-field imaging through dielectric microspheres has emerged in recent years as a simple and effective approach for generating super-resolution images at visible wavelengths. We present, to our knowledge, the first demonstration that dielectric microspheres can be used in a wide-field infrared (IR) microscope to enhance the far field resolution. We have observed a substantial improvement in resolution and magnification when images are collected through polystyrene microspheres. In addition, we demonstrate that spectroscopic imaging with a pulse-shaper based femtosecond mid-IR laser system is possible through the dielectric microspheres, which is a promising first step toward applying this technique to ultrafast IR imaging methods such as pump-probe and 2DIR microscopy.
引用
收藏
页码:5534 / 5541
页数:8
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