Study of flow channel geometry using current distribution measurement in a high temperature polymer electrolyte membrane fuel cell

被引:64
|
作者
Lobato, Justo [1 ]
Canizares, Pablo [1 ]
Rodrigo, Manuel A. [1 ]
Javier Pinar, F. [1 ]
Ubeda, Diego [1 ]
机构
[1] Univ Castilla La Mancha, Dept Chem Engn, E-13071 Ciudad Real, Spain
关键词
Channel geometry; PBI; Current distribution; High temperature PEMFC; OPERATIONAL PARAMETERS; DIAGNOSTIC-TOOLS; CATALYTIC LAYER; PERFORMANCE; DESIGN;
D O I
10.1016/j.jpowsour.2010.10.017
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
To improve fuel cell design and performance, research studies supported by a wide variety of physical and electrochemical methods have to be carried out. Among the different techniques, current distribution measurement owns the desired feature that can be performed during operation, revealing information about internal phenomena when the fuel cell is working. Moreover, short durability is one of the main problems that is hindering fuel cell wide implementation and it is known to be related to current density heterogeneities over the electrode surface. A good flow channel geometry design can favor a uniform current density profile, hence hypothetically extending fuel cell life. With this, it was thought that a study on the influence of flow channel geometry on the performance of a high temperature polymer electrolyte membrane (PEM) fuel cell using current distribution measurement should be a very solid work to optimize flow field design. Results demonstrate that the 4 step serpentine and pin-type geometries distribute the reactants more effectively, obtaining a relatively flat current density map at higher current densities than parallel or interdigitated ones and yielding maximum powers up to 25% higher when using oxygen as comburent. If air is the oxidant chosen, interdigitated flow channels perform almost as well as serpentine or pin-type due to that the flow conditions are very important for this geometry. (C) 2010 Elsevier B.V. All rights reserved.
引用
收藏
页码:4209 / 4217
页数:9
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