Rapid carbon mineralization for permanent disposal of anthropogenic carbon dioxide emissions

被引:579
|
作者
Matter, Juerg M. [1 ,2 ]
Stute, Martin [2 ]
Snaebjornsdottir, Sandra O. [3 ]
Oelkers, Eric H. [3 ,4 ,5 ]
Gislason, Sigurdur R. [3 ]
Aradottir, Edda S. [6 ]
Sigfusson, Bergur [6 ,7 ]
Gunnarsson, Ingvi [6 ]
Sigurdardottir, Holmfridur [6 ]
Gunnlaugsson, Einar [6 ]
Axelsson, Gudni [8 ]
Alfredsson, Helgi A. [3 ]
Wolff-Boenisch, Domenik [3 ,9 ]
Mesfin, Kiflom [3 ]
Taya, Diana Fernandez De la Reguera [2 ]
Hall, Jennifer [2 ]
Dideriksen, Knud [10 ]
Broecker, Wallace S. [2 ]
机构
[1] Univ Southampton, Dept Ocean & Earth Sci, Southampton, Hants, England
[2] Columbia Univ, Lamont Doherty Earth Observ, Palisades, NY USA
[3] Univ Iceland, Inst Earth Sci, IS-101 Reykjavik, Iceland
[4] Univ Toulouse 3, CNRS, UMR 5563, F-31062 Toulouse, France
[5] UCL, Dept Earth Sci, London WC1E 6BT, England
[6] Reykjavik Energy, Reykjavik, Iceland
[7] European Commiss, Joint Res Ctr, Inst Energy & Transport, Petten, Netherlands
[8] Iceland GeoSurvey, Reykjavik, Iceland
[9] Curtin Univ, Dept Appl Geol, Perth, WA 6845, Australia
[10] Univ Copenhagen, Dept Chem, Nanosci Ctr, DK-2100 Copenhagen, Denmark
关键词
GEOLOGICAL RESERVOIRS; STORAGE; SEQUESTRATION; LEAKAGE; HELLISHEIDI; CAPTURE; WATER; FIELD;
D O I
10.1126/science.aad8132
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Carbon capture and storage (CCS) provides a solution toward decarbonization of the global economy. The success of this solution depends on the ability to safely and permanently store CO2. This study demonstrates for the first time the permanent disposal of CO2 as environmentally benign carbonate minerals in basaltic rocks. We find that over 95% of the CO2 injected into the CarbFix site in Iceland was mineralized to carbonate minerals in less than 2 years. This result contrastswith the common view that the immobilization of CO2 as carbonate minerals within geologic reservoirs takes several hundreds to thousands of years. Our results, therefore, demonstrate that the safe long-term storage of anthropogenic CO2 emissions through mineralization can be far faster than previously postulated.
引用
收藏
页码:1312 / 1314
页数:3
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