Impact of biomass burning on a metropolitan area in the Amazon during the 2015 El Nino: The enhancement of carbon monoxide and levoglucosan concentrations

被引:15
|
作者
Ribeiro, Igor O. [1 ]
do Santos, Erickson O. [2 ]
Batista, Carla E. [1 ]
Fernandes, Karenn S. [2 ]
Ye, Jianhuai [3 ]
Medeiros, Adan S. [4 ]
Oliveira, Rafael L. E. [4 ]
de Sa, Suzane S. [3 ]
de Sousa, Thaiane R. [5 ]
Kayano, Mary T. [6 ]
Andreoli, Rita, V [4 ]
Machado, Cristine de M. D. [2 ]
Surratt, Jason D. [7 ]
Junior, Sergio D. [4 ]
Martin, Scot T. [3 ]
de Souza, Rodrigo A. F. [4 ]
机构
[1] INPA UEA, CLIAMB, Postgrad Program Climate & Environm, Av Andre Araujo 2936,Campus 2, BR-69060001 Manaus, Amazonas, Brazil
[2] Univ Fed Amazonas, Dept Chem, Av Gen Rodrigo Octavio Jordao Ramos 1200, BR-69067005 Manaus, Amazonas, Brazil
[3] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA
[4] Univ Amazonas State, Super Sch Technol, Av Darcy Vargas 1200,Parque 10 Novembro, BR-69065020 Manaus, Amazonas, Brazil
[5] INPA, PPG ECO, Postgrad Program Ecol, Av Andre Araujo 97,Campus 3, BR-69060000 Manaus, Amazonas, Brazil
[6] Natl Inst Space Res, Ctr Weather Forecasting & Climate Res, Av Astronautas 1758, BR-12227010 Sao Jose Dos Campos, SP, Brazil
[7] Univ N Carolina, Dept Environm Sci & Engn, Chapel Hill, NC 27516 USA
关键词
Amazon drought; El Nino Southern Oscillation; Air pollution; Forest fire; Manaus; GLOBAL FIRE EMISSIONS; ATMOSPHERIC AEROSOLS; MONOSACCHARIDE ANHYDRIDES; PARTICULATE MATTER; ORGANIC AEROSOLS; CLIMATE-CHANGE; HUMAN HEALTH; AIR-QUALITY; LAND-USE; DEFORESTATION;
D O I
10.1016/j.envpol.2020.114029
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Extreme droughts associated with changes in the climate have occurred every 5 years in the Amazon during the 21st century, with the most severe being in 2015. The increase in biomass burning (BB) events that occurred during the 2015 drought had several negative socioeconomic and environmental impacts, one of which was a decrease in the air quality. This study is an investigation into the air quality in the Manaus Metropolitan Region (MMR) (central Amazon, Brazil) during the dry (September to October) and wet (April to May) seasons of 2015 and 2016. A strong El Nino event began during the wet season of 2015 and ended during the wet season of 2016. Particulate matter samples were collected in the MMR during 2015 and 2016, and analyses of the satellite-estimated total carbon monoxide (CO) column and observed levoglucosan concentrations were carried out. Levoglucosan has been shown to be significantly correlated with regional fires and is a well-established chemical tracer for the atmospheric particulates emitted by BB, and CO can be treated as a gaseous-phase tracer for BB. The number of BB events increased significantly during the El Nino period when compared to the average number during 2003 -2016. Consequently, the total CO column and levoglucosan concentration values in the MMR increased by 15% and 500%, respectively, when compared to the normal conditions. These results indicate that during the period that was analyzed, the impacts of BB were exacerbated during the strong El Nino event as compared to the non-El Nino period. In this study, we provided evidence that the air quality in the MMR will degrade in the future if droughts and BB occurrences continue to increase. (C) 2020 Elsevier Ltd. All rights reserved.
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页数:10
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