Separation of cesium from wastewater with copper hexacyanoferrate film in an electrochemical system driven by microbial fuel cells

被引:26
|
作者
Tao, Qinqin [1 ,2 ]
Zhang, Xu [2 ]
Prabaharan, Krishnamoorthy [1 ]
Dai, Ying [1 ]
机构
[1] East China Univ Technol, State Key Lab Nucl Resources & Environm, Nanchang 330013, Jiangxi, Peoples R China
[2] East China Jiaotong Univ, Sch Civil Engineer & Architecture, Nanchang 330013, Jiangxi, Peoples R China
基金
中国国家自然科学基金;
关键词
Electrochemical; Adsorption; Copper hexacyanoferrate; Cesium; Microbial fuel cell; RADIOACTIVE CESIUM; ION-EXCHANGE; REMOVAL; ELECTRICITY; GENERATION; ADSORPTION;
D O I
10.1016/j.biortech.2019.01.093
中图分类号
S2 [农业工程];
学科分类号
0828 ;
摘要
A electrochemical adsorption system driven by microbial fuel cell (MFC-adsorption) was developed based on copper(II) hexacyanoferrate(III) (CuHCF) film for cesium (Cs) removal from wastewater. Cs uptake and elution can be simply controlled by regulating the redox states of the CuHCF films. Chemical oxygen demand (COD) removal showed little difference as MFC was connected to adsorption system. Meanwhile, power density and coulombic efficiency of MFC were dramatically reduced. The efficiencies of Cs adsorption and desorption were undesirable. MFC-adsorption technology used for actual nuclear wastewater treatment still has far to go.
引用
收藏
页码:456 / 459
页数:4
相关论文
共 50 条
  • [1] Column study on electrochemical separation of cesium ions from wastewater using copper hexacyanoferrate film
    Rongzhi Chen
    Miyuki Asai
    Chikako Fukushima
    Manabu Ishizaki
    Masato Kurihara
    Makoto Arisaka
    Takuya Nankawa
    Masayuki Watanabe
    Tohru Kawamoto
    Hisashi Tanaka
    Journal of Radioanalytical and Nuclear Chemistry, 2015, 303 : 1491 - 1495
  • [2] Column study on electrochemical separation of cesium ions from wastewater using copper hexacyanoferrate film
    Chen, Rongzhi
    Asai, Miyuki
    Fukushima, Chikako
    Ishizaki, Manabu
    Kurihara, Masato
    Arisaka, Makoto
    Nankawa, Takuya
    Watanabe, Masayuki
    Kawamoto, Tohru
    Tanaka, Hisashi
    JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY, 2015, 303 (02) : 1491 - 1495
  • [3] Preparation of a film of copper hexacyanoferrate nanoparticles for electrochemical removal of cesium from radioactive wastewater
    Chen, Rongzhi
    Tanaka, Hisashi
    Kawamoto, Tohru
    Asai, Miyuki
    Fukushima, Chikako
    Kurihara, Masato
    Watanabe, Masayuki
    Arisaka, Makoto
    Nankawa, Takuya
    ELECTROCHEMISTRY COMMUNICATIONS, 2012, 25 : 23 - 25
  • [4] Selective removal of cesium ions from wastewater using copper hexacyanoferrate nanofilms in an electrochemical system
    Chen, Rongzhi
    Tanaka, Hisashi
    Kawamoto, Tohru
    Asai, Miyuki
    Fukushima, Chikako
    Na, Haitao
    Kurihara, Masato
    Watanabe, Masayuki
    Arisaka, Makoto
    Nankawa, Takuya
    ELECTROCHIMICA ACTA, 2013, 87 : 119 - 125
  • [5] Removal of cesium from aqueous solutions by copper hexacyanoferrate membrane coated electrodes in a electrochemical adsorption system
    Chen, R. Z.
    Tanaka, H.
    Kawamoto, T.
    Asai, M.
    Fukushima, C.
    Watanabe, M.
    Kurihara, M.
    Arisaka, M.
    Nankawa, T.
    EUROMEMBRANE CONFERENCE 2012, 2012, 44 : 1728 - 1730
  • [6] Thermodynamics and Mechanism Studies on Electrochemical Removal of Cesium Ions from Aqueous Solution Using a Nanoparticle Film of Copper Hexacyanoferrate
    Chen, Rongzhi
    Tanaka, Hisashi
    Kawamoto, Tohru
    Asai, Miyuki
    Fukushima, Chikako
    Kurihara, Masato
    Ishizaki, Manabu
    Watanabe, Masayuki
    Arisaka, Makoto
    Nankawa, Takuya
    ACS APPLIED MATERIALS & INTERFACES, 2013, 5 (24) : 12984 - 12990
  • [7] High efficiency electrochemical separation of uranium(VI) from uranium-containing wastewater by microbial fuel cells with different cathodes
    Sun, Du
    Lv, Chunxue
    Hua, Yilong
    Li, Mi
    Zhang, Xiaowen
    Fang, Qi
    Cai, Tao
    Wu, Xiaoyan
    BIOELECTROCHEMISTRY, 2023, 151
  • [8] Selective separation of cesium from radioactive liquid waste by potassium copper hexacyanoferrate (II)-clinoptilolite composite
    Ri, Song-Hyok
    Kim, Yong-Nam
    Im, Sun-Jong
    Choe, Song-Gun
    Kim, Chol-Hyok
    JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY, 2023, 332 (06) : 2329 - 2337
  • [9] Selective separation of cesium from radioactive liquid waste by potassium copper hexacyanoferrate (II)-clinoptilolite composite
    Song-Hyok Ri
    Yong-Nam Kim
    Sun-Jong Im
    Song-Gun Choe
    Chol-Hyok Kim
    Journal of Radioanalytical and Nuclear Chemistry, 2023, 332 : 2329 - 2337
  • [10] Electrochemical Insight into the Use of Microbial Fuel Cells for Bioelectricity Generation and Wastewater Treatment
    Tabish, Asif Nadeem
    Farhat, Iqra
    Irshad, Muneeb
    Hussain, Muhammad Asif
    Usman, Muhammad
    Chaudhary, Tariq Nawaz
    Fouad, Yasser
    Raza, Sohaib
    Ashraf, Waqar Muhammad
    Krzywanski, Jaroslaw
    ENERGIES, 2023, 16 (06)