Photocatalytic CO2 reduction using visible light by metal-monocatecholato species in a metal-organic framework

被引：104

作者：

Lee, Yeob ^{[1
]}

Kim, Sangjun ^{[2
]}

Fei, Honghan ^{[1
]}

Kang, Jeung Ku ^{[2
]}

Cohen, Seth M. ^{[1
]}

机构：

[1] Univ Calif San Diego, Dept Chem & Biochem, San Diego, CA 92093 USA

[2] Korea Adv Inst Sci & Technol, Grad Sch EEWS, Taejon 305701, South Korea

来源：

CHEMICAL COMMUNICATIONS | 2015年 / 51卷 / 92期

关键词：

CARBON-DIOXIDE; HYDROGEN-PRODUCTION; POSTSYNTHETIC LIGAND; COMPLEXES; CATALYSIS; EXCHANGE; FUNCTIONALIZATION; OXIDATION; ENERGY;

D O I：

10.1039/c5cc04506a

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Metal-organic frameworks (MOFs) with isolated metal-monocatecholato groups have been synthesized via postsynthetic exchange (PSE) for CO2 reduction photocatalyst under visible light irradiation in the presence of 1-benzyl-1,4-dihydronicotinamide and triethanolamine. The Cr-monocatecholato species are more efficient than the Ga-monocatecholato species.

引用

页码：16549 / 16552

页数：4

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