Dibenzoarsacrowns: an experimental and computational study on the coordination behaviors

被引：6

作者：

Sumida, Akifumi ^{[1
]}

Kobayashi, Ryosuke ^{[1
]}

Yumura, Takashi ^{[2
]}

Imoto, Hiroaki ^{[1
,3
]}

Naka, Kensuke ^{[1
,3
]}

机构：

[1] Kyoto Inst Technol, Fac Mol Chem & Engn, Sakyo Ku, Goshokaido Cho, Kyoto 6068585, Japan

[2] Kyoto Inst Technol, Fac Mat Sci & Technol, Sakyo Ku, Goshokaido Cho, Kyoto 6068585, Japan

[3] Kyoto Inst Technol, Mat Innovat Lab, Sakyo Ku, Goshokaido Cho, Kyoto 6068585, Japan

来源：

CHEMICAL COMMUNICATIONS | 2021年 / 57卷 / 16期

关键词：

D O I：

10.1039/d0cc07191a

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Dibenzoarsacrowns have been synthesized as a novel class of heteroatom-fused crown ethers. The dibenzoarsacrowns can size-selectively capture alkali metal cations, and the arsenic atoms chemoselectively coordinated to gold(I) chloride (AuCl) due to the soft Lewis acid-base interaction. It is notable that the AuCl complex of 21-dibenzoarsacrown-7 further encapsulated Na+ with the enhanced association constant from bare 21-dibenzoarsacrown-7. The positive allosteric effect was studied computationally.

引用

页码：2013 / 2016

页数：4

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