Heterogeneous Palladium Catalysts for Decarbonylation of Biomass-Derived Molecules under Mild Conditions

被引：72
|
作者：
Huang, Yao-Bing [1 ]
Yang, Zhen [1 ]
Chen, Meng-Yuan [1 ]
Dai, Jian-Jun [1 ]
Guo, Qing-Xiang [1 ]
Fu, Yao [1 ]
机构：
[1] Univ Sci & Technol China, Dept Chem, Anhui Prov Key Lab Biomass Clean Energy, Hefei 230026, Peoples R China
来源：
CHEMSUSCHEM | 2013年 / 6卷 / 08期
关键词：
biomass conversion; decarbonylations; heterogeneous catalysis; 5-hydroxymethylfurfural; palladium; SELECTIVE DECARBONYLATION; TRANSFER HYDROGENATION; LEVULINIC ACID; FUELS; CONVERSION; ALDEHYDES; ALKANES; TRANSFORMATION; DECOMPOSITION; CELLULOSE;
D O I：
10.1002/cssc.201300190
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
Workin′ 6 to 5: A highly active heterogeneous catalyst, Pd/SBA-15(DP), promotes the selective decarbonylation of biomass-derived HMF to furfural alcohol with a high yield, up to 96 %, in mild conditions. The route offers a simple and effective method of linking C6 and C5 molecules in the biomass conversion value chain. In addition to HMF the catalyst is effective towards the decarbonylation of other biomass-derived aldehydes, also. Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
引用
收藏
页码：1348 / 1351
页数：4
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