Oxy-fuel conversion of sub-bituminous coal particles in fluidized bed and pulverized combustors

被引:23
|
作者
Bu, Changsheng [1 ,2 ]
Gomez-Barea, Alberto [3 ]
Leckner, Bo [4 ]
Chen, Xiaoping [2 ]
Pallares, David [4 ]
Liu, Daoyin [2 ]
Lu, Ping [1 ]
机构
[1] Nanjing Normal Univ, Sch Energy & Mech Engn, Jiangsu Prov Key Lab Mat Cycling & Pollut Control, Nanjing 210042, Jiangsu, Peoples R China
[2] Southeast Univ, Key Lab Energy Thermal Convers & Control, Minist Educ, Nanjing 210096, Jiangsu, Peoples R China
[3] Univ Seville, Chem & Environm Engn Dept, Seville 41092, Spain
[4] Chalmers, Environm & Energy Dept, S-41296 Gothenburg, Sweden
基金
中国博士后科学基金; 中国国家自然科学基金;
关键词
Fluidized bed; Pulverized coal; Oxy-fuel combustion; Sub-bituminous coal; CO2 GASIFICATION REACTION; CHAR PARTICLES; O-2/CO2; ATMOSPHERES; CONDITIONS; PART; HEAT-TRANSFER; DEVOLATILIZATION; IGNITION; O-2/N-2; TEMPERATURE; BEHAVIOR;
D O I
10.1016/j.proci.2016.08.075
中图分类号
O414.1 [热力学];
学科分类号
摘要
Oxy-fuel combustion in pulverized coal (PC) and fluidized bed (FB) boilers is being increasingly investigated due to its potential use for carbon dioxide capture. The combustion conditions in the two types of unit differ significantly because of fuel size, furnace temperature, and fluid dynamics. These differences affect the change of combustion characteristics from air (O-2/N-2) to oxy-fuel (O-2/CO2) conditions in PC and FB in different ways. In this paper, the oxy-fuel combustion behavior of a single sub-bituminous coal particle in PC is compared with that in FB conditions. The FB data were measured in our bench-scale FB test rig, whereas the PC data were collected from literature. The FB tests were performed at 1088 K with 0%(vol) < O-2 < 40%(vol), using sub-bituminous coal with a diameter of 6 mm. An extensive list of parameters is compared, including the ignition-delay time, volatiles' flame temperature, devolatilization time, burnout time and peak temperature of the coal particle. Results indicate that the impact of shifting from air-firing to oxy-firing af-fects the devolatilization, burnout times, and peak temperature in PC and FB differently: PC particles require higher concentration of oxygen than coarse particles for FB to attain similar results as in air-firing. However, the impact on the volatile flame temperature of shifting to oxy-fuel flame is similar in PC and FB. In general, the CO2 atmosphere delays ignition compared to air-firing, particularly for coarse particles at low O-2 concentration. (C) 2016 by The Combustion Institute. Published by Elsevier Inc.
引用
收藏
页码:3331 / 3339
页数:9
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