Natural Gas to Fuels and Chemicals: Improved Methane Aromatization in an Oxygen-Permeable Membrane Reactor

被引：91
|
作者：
Cao, Zhengwen [1 ]
Jiang, Heqing [2 ]
Luo, Huixia [1 ,3 ]
Baumann, Stefan [4 ]
Meulenberg, Wilhelm A. [4 ]
Assmann, Jens [5 ]
Mleczko, Leslaw [5 ]
Liu, Yi [1 ]
Caro, Juergen [1 ]
机构：
[1] Leibniz Univ Hannover, Inst Phys Chem & Electrochem, D-30167 Hannover, Germany
[2] Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Key Lab Biobased Mat, Qingdao 266101, Peoples R China
[3] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA
[4] Forschungszentrum Julich GmbH, Inst Energy & Climate Res, D-52425 Julich, Germany
[5] Bayer Technol Serv GmbH, BTS TD UP Chem Catalysis, D-51368 Leverkusen, Germany
来源：
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION | 2013年 / 52卷 / 51期
关键词：
aromatic compounds; dehydroaromatization; membrane reactors; methane; oxygen-permeable membranes; NONOXIDATIVE ACTIVATION; CATALYTIC PERFORMANCE; HYDROGEN-PRODUCTION; WATER DISSOCIATION; CONVERSION; MO/HZSM-5; PEROVSKITE; DEHYDROAROMATIZATION; DEHYDROGENATION; REDUCTION;
D O I：
10.1002/anie.201307935
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
Adding value with membranes: Improved methane aromatization was achieved by using an oxygen-permeable membrane. The resulting membrane reactor shows a superior methane conversion and a higher resistance towards catalyst deactivation. Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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页码：13794 / 13797
页数：4
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