A method for quick assessment of CO2 storage capacity in closed and semi-closed saline formations

被引:330
|
作者
Zhou, Quanlin [1 ]
Birkholzer, Jens T. [1 ]
Tsang, Chin-Fu [1 ]
Rutqvist, Jonny [1 ]
机构
[1] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Earth Sci, Berkeley, CA 94720 USA
关键词
Geological CO2 sequestration; Storage capacity; Saline aquifer; Pressure buildup; Numerical simulation;
D O I
10.1016/j.ijggc.2008.02.004
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Saline aquifers of high permeability bounded by overlying/underlying seals may be surrounded laterally by low-permeability zones, possibly caused by natural heterogeneity and/or faulting. Carbon dioxide (CO2) injection into and storage in such "closed" systems with impervious seals, or "semi-closed" systems with non-ideal (low permeability) seals, is different from that in "open" systems, from which the displaced brine can easily escape laterally. in closed or semi-closed systems, the pressure buildup caused by continuous industrial-scale CO2 injection may have a limiting effect on CO2 storage capacity, because geomechanical damage caused by overpressure needs to be avoided. In this research, a simple analytical method was developed for the quick assessment of the CO2 storage capacity in such closed and semi-closed systems. This quick-assessment method is based on the fact that native brine (of an equivalent volume) displaced by the cumulative injected CO2 occupies additional pore volume within the storage formation and the seals, provided by pore and brine compressibility in response to pressure buildup. With non-ideal seals, brine may also leak through the seals into overlying/underlying formations. The quick-assessment method calculates these brine displacement contributions in response to an estimated average pressure buildup in the storage reservoir. The CO2 storage capacity and the transient domain-averaged pressure buildup estimated through the quick-assessment method were compared with the "true" values obtained using detailed numerical simulations of CO2 and brine transport in a two-dimensional radial system. The good agreement indicates that the proposed method can produce reasonable approximations for storage-formation-seal systems of various geometric and hydrogeological properties. (C) 2008 Elsevier Ltd. All rights reserved.
引用
收藏
页码:626 / 639
页数:14
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