Inorganic-organic photocatalyst BiPO4/g-C3N4 for efficient removal of gaseous toluene under visible light irradiation

被引:39
|
作者
Zou, Xuejun [1 ]
Dong, Yuying [1 ]
Li, Xinyong [2 ,3 ]
Zhao, Qidong [2 ,3 ]
Cui, Yubo [1 ]
Lu, Guang [4 ]
机构
[1] Dalian Nationalities Univ, Dept Environm Sci & Technol, Dalian 116600, Peoples R China
[2] Dalian Univ Technol, Sch Environm Sci & Technol, State Key Lab Fine Chem, Dalian 116024, Peoples R China
[3] Dalian Univ Technol, Sch Environm Sci & Technol, Key Lab Ind Ecol & Environm Engn, Dalian 116024, Peoples R China
[4] Liaoning Shihua Univ, Coll Chem Chem Engn & Environm Engn, Fushun 113001, Peoples R China
关键词
BiPO4/g-C3N4; Photocatalytic oxidation; Toluene; Nanocomposites; HYDROGEN-PRODUCTION; MESOPOROUS G-C3N4; DEGRADATION; CONVERSION;
D O I
10.1016/j.catcom.2015.04.035
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
BiPO4/g-C3N4 with different amounts of BiPO4 was prepared through wet impregnation with calcination method. The BiPO4/g-C3N4 showed large surface area (172.9 m(2) g(-1)) and the incorporation of BiPO4 caused a red-shift of g-C3N4 in visible light. The photocatalytic degradation of toluene over the samples was investigated. The degradation of toluene could get 82% in BiPO4/g-C3N4 photocatalysts under optimum reaction conditions. The BiPO4/g-C3N4 exhibited a higher photocatalytic activity than pure g-C3N4 or BiPO4. The improved photoactivity of BiPO4/g-C3N4 could be attributed to strong absorption in visible light and effective separation of photoinduced hole-electron pairs between BiPO4 and g-C3N4. (C) 2015 Elsevier B.V. All rights reserved.
引用
收藏
页码:109 / 113
页数:5
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