Measurements of aerosol number concentrations and rainwater chemistry at Mt. Tateyama, near the coast of the Japan sea in central Japan: On the influence of high-elevation Asian dust particles in autumn

Measurements of size-separated aerosol number concentrations at Midagahara (altitude, 1,930 m), on the western slope of Mt. Tateyama near the coast of the Japan Sea, were performed each autumn from 2006 to 2011. High number concentrations of particles larger than 2 mu m were frequently seen in 2006 and 2009 when the influence of Asian dust might have been significant. The pH and the ratio of Ca2+ to total ions were high in the rainwater bulk sampled when high number concentrations of coarse particles were observed. The mean pH of rainwater during the autumn in 2006 was significantly higher than that in 2007 and 2008. Acidic species might have been neutralized by the Asian dust particles. Dust particles may highly affect the natural environment, such as forest ecosystems, at high elevations during seasons without snow cover.