Real-time observation of phase-controlled molecular wave-packet interference

被引：87
|
作者：
Ohmori, K [1 ]
Katsuki, H
Chiba, H
Honda, M
Hagihara, Y
Fujiwara, K
Sato, Y
Ueda, K
机构：
[1] Natl Inst Nat Sci, Inst Mol Sci, Okazaki, Aichi 4448585, Japan
[2] Grad Univ Adv Studies, Okazaki, Aichi 4448585, Japan
[3] Tohoku Univ, IMRAM, Sendai, Miyagi 9808577, Japan
[4] CREST, Japan Sci & Technol Agcy, Kawaguchi, Saitama 3320012, Japan
来源：
PHYSICAL REVIEW LETTERS | 2006年 / 96卷 / 09期
关键词：
D O I：
10.1103/PhysRevLett.96.093002
中图分类号：
O4 [物理学];
学科分类号：
0702 ;
摘要：
The quantum interference of two molecular wave packets has been precisely controlled in the B electronic state of the I-2 molecule by using a pair of fs laser pulses whose relative phase is locked within the attosecond time scale and its real-time evolution has been observed by another fs laser pulse. It is clearly observed that the temporal evolution changes drastically as a function of the relative phase between the locked pulses, allowing us to read both amplitude and phase information stored in the wave functions of the molecular ensemble.
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页数：4
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